期刊
ORGANIC LETTERS
卷 14, 期 14, 页码 3565-3567出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301481t
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资金
- European Research Council under the European Union [277588]
- European Research Council (ERC) [277588] Funding Source: European Research Council (ERC)
The first total synthesis of the paracaseolide A, a very unusual tetraquinane oxa-cage bislactone recently isolated from the mangrove Sonneratia paracaseolaris, has been achieved. The final step and culmination of the eight-step synthetic sequence is a [4 + 2] dimerization of a 4-hydroxybutenolide, generated by singlet oxygen-mediated oxidation of a furan precursor.
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