期刊
ORGANIC LETTERS
卷 14, 期 23, 页码 5868-5871出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol302757y
关键词
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资金
- JSPS
- MEXT, Japan
- Grants-in-Aid for Scientific Research [24790011, 24590035] Funding Source: KAKEN
A highly efficient short-step construction of the common phenanthridine skeleton of pancratistatin-class alkaloids was accomplished in enantiomerically pure form using chiral ligand-controlled asymmetric conjugate addition. The utility of the intermediate was demonstrated by the total synthesis of (+)-trans-dihydronarciclasine with mild oxidation from an amine to an amide as a key step.
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