期刊
ORGANIC LETTERS
卷 14, 期 6, 页码 1516-1519出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol3002514
关键词
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资金
- Aarhus University
- Carlsberg Foundation
- FNU
An enantioselective synthesis of gamma-nitroesters by a one-pot asymmetric Michael addition/oxidative esterification of alpha,beta-unsaturated aldehydes is presented. The procedure is based on merging the enantioselective organocatalytic nitroalkane addition with an N-bromosuccinimide-based oxidation. The gamma-nitroesters are obtained in good yields and enantioselectivities, and the method provides an attractive entry to optically active gamma-aminoesters, 2-piperidones, and 2-pyrrolidones.
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