期刊
ORGANIC LETTERS
卷 14, 期 9, 页码 2293-2295出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol3007138
关键词
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资金
- MOST [2010CB833200]
- NSFC [21125207, 21072086, 21102062]
- program 111
A concise construction of the 6/6/5 tricyclic core of Lycopodium alkaloid palhinine A (1) has been accomplished. The developed synthetic strategy featured a tandem oxidative dearomatization/intramolecular Diels-Alder reaction to construct C/D rings and an intramolecular 5-exo-trig radical cyclization to install the B ring of palhinine A (1). The developed approach paves the way for the total synthesis of palhinine A (1).
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