期刊
ORGANIC LETTERS
卷 14, 期 13, 页码 3554-3557出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301618r
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资金
- Dalian Institute of Chemical Physics (CAS)
- Planned Science and Technology Project of Dalian [2011J21DW010]
A mild and general iridium-catalyzed, highly enantioselective hydrogenation of sterically hindered N-arylimines with a new H-8-BINOL-derived phosphine-phosphoramidite ligand has been developed. The present catalytic system features high turnover numbers (up to 100000) and good to perfect enantioselectivities (up to 99% ee) for the hydrogenation of a variety of sterically hindered N-arylimines.
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