期刊
ORGANIC LETTERS
卷 13, 期 2, 页码 336-339出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol102892f
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资金
- UPV/EHU
- MICINN [CTQ2008-00136/BQU]
- DFB/BFA [DIPE08/03]
- EJ/GV [Grupos IT328-10]
5-Mercaptotetrazoles have been identified as useful and versatile Michael donors in enantioselective amine-catalyzed aza-Michael reactions with alpha,beta-unsaturated aldehydes, showing excellent behavior as N-nucleophiles instead of their usual trend to react as S-nucleophiles. In addition several unprecedented chemical modifications on the tetrazolothione moiety have been carried out leading to the enantioselective preparation of different compounds incorporating nitrogen-containing functionalities such as oxazinimines, formamidines, ureas and isoureas.
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