期刊
ORGANIC LETTERS
卷 12, 期 12, 页码 2682-2685出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol1007795
关键词
-
资金
- Ministry of Education in Singapore [ARC12/07, T206B3225]
A highly enantio- and diastereoselective organocatalytic domino Michael Henry process for the preparation of synthetically unique and medicinally important bicyclo[3.2.1]octane derivatives with four stereogenic centers including two quaternary stereocenters has been developed. Theoretical OFT calculations on the transition states have been carried out to reveal origins of the excellent stereoselectivities. A novel dual model was thus proposed.
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