期刊
ORGANIC LETTERS
卷 11, 期 21, 页码 4778-4781出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol902097d
关键词
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资金
- MEC Spain [CTQ2007-61254/BQU, CTQ2008-01565/BQU]
- FPU fellowship
- Junta de Andalucia [FQM-345]
Efficient methodologies for the synthesis of regioisomeric 3-pyrrolines by reaction of electron-deficient imines and sulfur-containing allenyl derivatives are presented. Lithiated thioallenes give 2-aryl-3-phenylsulfonyl-3-pyrrolines, whereas allenyl sulfones furnish the isomeric 2-aryl-4-phenylsulfonyl-3-pyrrolines through migration of the sulfonyl group that catalyzes the nucleophilic [3 + 2] cycloaddition.
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