期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 10, 期 46, 页码 9237-9242出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob26586a
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资金
- NSFC [20972027, 21172034]
- Program for New Century Excellent Talents in University [NCET-11-0611]
- Department of Science and Technology of Jilin Province [201215002]
- Fundamental Research Funds for the Central Universities [11SSXT129]
- Open Project of State Key Laboratory of Supramolecular Structure and Materials [sklssm201225]
A simple, efficient and practical copper-catalyzed aerobic oxidative synthesis of alpha-ketoamides from aryl methyl ketones, aliphatic amines and N-iodosuccinimide (NIS) has been developed. The one-pot reaction may proceed smoothly at room temperature in the open air. The possible mechanism for the formation of a-ketoamides was proposed. Molecular oxygen in air functions as both an oxidant and an oxygen source.
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