期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 10, 期 25, 页码 4851-4863出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob25400j
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资金
- Oregon State University (OSU)
- National Science Foundation [CHE-0848704, CHE-0722319]
- Murdock Charitable Trust [2005265]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0848704] Funding Source: National Science Foundation
The development of a proline sulphonamide-catalysed method for enantioselective and diastereoselective construction of functionalized cyclohexenones is described. Impact of catalyst structure as well as solvent effects and additives are explored. A significant substrate scope is demonstrated by variation of both the aldehyde and the enone components. Diastereoselective derivatization of the cyclohexenone scaffold illustrates its utility as a building block for chemical synthesis.
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