期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 10, 期 30, 页码 5965-5970出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob25069a
关键词
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A modular total synthesis of the natural product (+)-varitriol (1) and seven analogs was achieved by using combined coinage metal catalysis. Starting from enynol 13, reagent-controlled introduction of stereogenic centers and efficient center-to-axis-to-center chirality transfer via alpha-hydroxyallene 5 afforded (+)-varitriol with 6.4% yield over 10 steps.
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