期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 9, 期 21, 页码 7547-7553出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1ob06147j
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资金
- Pembroke College, Cambridge
- University of Bath
- EPSRC
Three new N-desymmetrised naphthalenediimides (NDIs) are described, each containing one chiral and one achiral centre. The ability of such 'monochiral' NDIs to self-assemble into hydrogen-bonded helical nanotubes, to act as a sergeant in a 'sergeants-and-soldiers' system and to form a hexameric receptor for C-70 was examined. Small differences at the achiral centre were found to have significant effects on the supramolecular properties of the NDI. All three new NDIs form nanotubes that bind C-60, but with different efficiencies, and one is a better sergeant than any of the dichiral NDIs investigated to date.
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