期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 7, 期 19, 页码 4120-4127出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b910939k
关键词
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资金
- National Natural Science Foundation of China [20732003, 20602025]
- Ministry of Education [2007061009]
Organocatalysts containing primary-secondary diamines based on bispidine have been developed to catalyze the asymmetric Michael addition of ketones to alkylidene malonates and nitroalkenes. The corresponding products were obtained in high yields (up to 99%) with high diastereoselectivities (up to 99: 1) and high enantioselectivities (up to 97% ee) under mild conditions using either environmentally benign water as the solvent or no solvent.
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