4.6 Article

Local refractive index sensitivity of plasmonic nanoparticles

期刊

OPTICS EXPRESS
卷 19, 期 10, 页码 9213-9220

出版社

OPTICAL SOC AMER
DOI: 10.1364/OE.19.009213

关键词

-

类别

资金

  1. Academy of Sciences of the Czech Republic [KAN200670701]
  2. Ministry of Education, Youth and Sports [OC09058]
  3. COST Action [MP0803]
  4. European Science Foundation (ESF)

向作者/读者索取更多资源

We report on an experimental characterization of the sensitivity of localized surface plasmons (LSP) to local changes in the refractive index at a nanometer scale. The method is based on forming a polymer mask covering different well defined areas of metallic nanoparticles and measuring the extinction peak shifts associated with the local refractive index changes. Arrays of nanoparticles (nanorod chains) are prepared using electron beam lithography and the dielectric mask is aligned with respect to the nanoparticle array in a second lithographic step. Extinction peak shifts corresponding to different positions of the mask are measured and values for the local refractive index sensitivity are deduced. A deconvolution procedure is established and used to map the local sensitivity across the surface of nanoparticle based on measured data. The experimental results are shown to correspond well with theoretical simulations obtained using the finite-difference time-domain method. The results indicate that the sensitivity is strongly correlated with the profile of the LSP electric field. (C) 2011 Optical Society of America

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.6
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Physics, Applied

Multiscale modeling and analysis for high-fidelity interferometric scattering microscopy

Yong He, Shupei Lin, Hadrien Marc Louis Robert, Hong Li, Pu Zhang, Marek Piliarik, Xue-Wen Chen

Summary: This paper presents a theoretical framework of multiscale modeling and analysis for interferometric scattering microscopy (iSCAT), exploring the influence of sample shape, illumination, and detection schemes on interference contrast, and providing an explanation for the origin of interference phenomenon. Additionally, it investigates the point spread function of gold nanoparticles in a simplified cell environment.

JOURNAL OF PHYSICS D-APPLIED PHYSICS (2021)

Article Multidisciplinary Sciences

Fast photothermal spatial light modulation for quantitative phase imaging at the nanoscale

Hadrien M. L. Robert, Kristyna Holanova, Lukasz Bujak, Milan Vala, Verena Henrichs, Zdenek Lansky, Marek Piliarik

Summary: The study introduces a high-speed photothermal spatial light modulator capable of generating a step-like wavefront change without diffraction artifacts, used for quantitative phase imaging to capture nanometer-scale 3D displacements.

NATURE COMMUNICATIONS (2021)

Review Nanoscience & Nanotechnology

Advances and applications of nanophotonic biosensors

Hatice Altug, Sang-Hyun Oh, Stefan A. Maier, Jiri Homola

Summary: This Review presents the progresses in label-free nanophotonic biosensors based on photonic or dielectric surfaces and metasurfaces, and discusses their challenges and benefits in the fields of public health, well-being, and biosafety. Nanophotonic devices can control light and enhance light-matter interactions at subwavelength scales, offering exciting prospects for biosensing applications.

NATURE NANOTECHNOLOGY (2022)

Article Chemistry, Analytical

Plasmonic biosensor based on a gold nanostripe array for detection of microRNA related to myelodysplastic syndromes

Jiri Slaby, Marketa Bockova, Jiri Homola

Summary: A new optical biosensor based on gold nanostripes array excited surface plasmons is presented, with theoretical analysis showing its improved detection sensitivity compared to conventional surface plasmon resonance biosensors. Experimental validation of the theoretical model demonstrates high refractive index sensitivity and resolution of the nanoplasmonic sensor. Additionally, the biosensor successfully detects microRNA biomarkers at low concentrations, showcasing its potential for sensitive and specific biomolecular detection.

SENSORS AND ACTUATORS B-CHEMICAL (2021)

Article Biochemistry & Molecular Biology

Anchored linear oligonucleotides: the effective tool for the real-time measurement of uracil DNA glycosylase activity

Anna Ligasova, Ivan Rosenberg, Marketa Bockova, Jiri Homola, Karel Koberna

Summary: This study introduces a novel approach for real-time measurement of uracil DNA glycosylase activity by immobilizing selected oligonucleotides on magnetic nanoparticles and utilizing Forster resonance energy transfer. The results demonstrate that this method provides more reliable data than using free oligonucleotides, and offers the possibility to investigate the relationship between uracil DNA glycosylase activity and the arrangement of oligonucleotide probes. Additionally, introducing a nick into oligonucleotides containing the target base (uracil) significantly decreases the activity of both bacterial glycosylase and glycosylases naturally present in nuclear lysates.

OPEN BIOLOGY (2021)

Article Physics, Multidisciplinary

Anomalous elasticity and damping in covalently cross-linked graphene aerogels

Martin Silhavik, Prabhat Kumar, Zahid Ali Zafar, Martin Misek, Martin Cicala, Marek Piliarik, Jiri Cervenka

Summary: Graphene aerogel exhibits anomalous superelastic behavior and can withstand high compressive and tensile strains. A quantitative origami model is developed to describe its stress-strain behavior.

COMMUNICATIONS PHYSICS (2022)

Article Chemistry, Multidisciplinary

Nonadiabatic Nano-optical Tunneling of Photoelectrons in Plasmonic Near-Fields

Bela Lovasz, Peter Sandor, Gellert-Zsolt Kiss, Balazs Banhegyi, Peter Racz, Zsuzsanna Papa, Judit Budai, Christine Prietl, Joachim R. Krenn, Peter Dombi

Summary: This study explores nonadiabatic nano-optical electron tunneling in the transition region between multiphoton-induced emission and adiabatic tunnel emission in the near-field of plasmonic nanostructures. The measured photoemission spectra exhibit strong-field recollision driven by the nanoscale near-field for Keldysh gamma values between approximately 1.3 and approximately 2.2. At the same time, the photoemission yield shows a constant nonlinearity in intensity scaling, which is characteristic of multiphoton-induced emission.

NANO LETTERS (2022)

Article Materials Science, Multidisciplinary

Multipitched plasmonic nanoparticle grating for broadband light enhancement in white light-emitting organic diodes

Manuel Auer-Berger, Veronika Tretnak, Christian Sommer, Franz-Peter Wenzl, Joachim R. Krenn, Emil J. W. List-Kratochvil

Summary: The study utilizes plasmonic nanodisk arrays to enhance light emission from an organic white light-emitting diode. By incorporating aluminum as the nanodisk material and employing surface lattice resonances from a multipitch array, the broadband enhancement of light emission in the device is achieved. The experimental results align well with simulations, providing insights into the underlying physical mechanisms.

APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING (2022)

Article Materials Science, Multidisciplinary

Shaping of Optical Wavefronts Using Light-Patterned Photothermal Metamaterial

Hadrien M. L. Robert, Martin Cicala, Marek Piliarik

Summary: Having full control of light propagation is the ultimate goal of an imaging system. The introduction of a photothermally modulated SLM allows for the generation of arbitrarily shaped wavefront patterns with high responsiveness and unique advantages, such as fast response, absence of diffraction artifacts, and high transmittance.

ADVANCED OPTICAL MATERIALS (2022)

Article Biophysics

Performance of label-free optical biosensors: What is figure of merit (not) telling us?

Jiri Slaby, Jiri Homola

Summary: In this study, we analyze the performance of label-free optical biosensors in detecting analyte-induced refractive index changes. We propose an analytical model that relates the refractive index resolution to the parameters of the optical platform. Our findings demonstrate that the widely used figure of merit (FOM) is not suitable for guiding the design or predicting the performance of label-free optical biosensors. Therefore, we propose an extended definition of FOM to address its limitations. The validity of our approach is confirmed through numerical simulations and experiments, and we show that the analytical model not only predicts the performance of biosensors but also provides strategies for achieving optimal performance.

BIOSENSORS & BIOELECTRONICS (2022)

Article Physics, Multidisciplinary

Optical Fingerprint of Flat Substrate Surface and Marker-Free Lateral Displacement Detection with Angstrom-Level Precision

Shupei Lin, Yong He, Delong Feng, Marek Piliarik, Xue-Wen Chen

Summary: We discovered that flat substrates with subnanometer surface undulations show notable speckle patterns when observed with high-sensitivity interference microscopy. We introduced the concept of optical fingerprints and demonstrated their use in position identification and displacement detection.

PHYSICAL REVIEW LETTERS (2022)

Article Engineering, Electrical & Electronic

Gain and lasing from CdSe/CdS nanoplatelet stripe waveguides

Martin Belitsch, Dmitry N. Dirin, Maksym V. Kovalenko, Kevin Pichler, Stefan Rotter, Ahmed Ghalgaoui, Harald Ditlbacher, Andreas Hohenau, Joachim R. Krenn

Summary: The study demonstrates the feasibility of using geometrically simple monolithic microscale CdSe/CdS nanoplatelet lasers as a promising option for various photonic applications. The CdSe/CdS nanoplatelets show high gain factor and emission pulse shortening.

MICRO AND NANO ENGINEERING (2022)

Proceedings Paper Nanoscience & Nanotechnology

Nonadiabatic nano-optical tunneling of photoelectrons in plasmonic near-fields

Bela Lovasz, Peter Sandor, Gellert-Zsolt Kiss, Balazs Banhegyi, Peter Racz, Zsuzsanna Papa, Judit Budai, Christine Prietl, Joachim R. Krenn, Peter Dombi

Summary: Our work demonstrates nonadiabatic tunneling of photoelectrons in the near-field of gold nanostructures, and investigates its characteristics in the transition region between the multi-photon-induced photoemission and tunneling emission regimes.

NANOPHOTONICS IX (2022)

Article Chemistry, Multidisciplinary

Photoconductivity of PbS/perovskite quantum dots in gold nanogaps

Dario Grimaldi, Emil Kelderer, Dmitry N. Dirin, Maksym Kovalenko, Andreas Hohenau, Harald Ditlbacher, Joachim R. Krenn

Summary: This study demonstrates that the photoconductance of colloidal PbS/MAPbI(3) quantum dots in nanoscale gold electrode gaps exhibits a power law dependence on the light intensity. The research reveals the strong localization and high reproducibility of photocurrent generation, and shows that different geometries and excitation methods yield practically identical photocurrent responses.

NANOSCALE ADVANCES (2022)

Article Polymer Science

Grafting density and antifouling properties of poly[N-(2-hydroxypropyl) methacrylamide] brushes prepared by grafting to and grafting from

Yu-Min Wang, Anna Kalosi, Yuriy Halahovets, Iryna Romanenko, Jiri Slaby, Jiri Homola, Jan Svoboda, Andres de los Santos Pereira, Ognen Pop-Georgievski

Summary: This study compared the anti-fouling properties of poly(HPMA) brushes prepared by chemisorption and surface-initiated polymerization methods, finding that the latter exhibited better anti-fouling performance due to higher grafting density.

POLYMER CHEMISTRY (2022)

暂无数据