4.8 Article

Superinsulator and quantum synchronization

期刊

NATURE
卷 452, 期 7187, 页码 613-U5

出版社

NATURE PUBLISHING GROUP
DOI: 10.1038/nature06837

关键词

-

向作者/读者索取更多资源

Synchronized oscillators are ubiquitous in nature(1), and synchronization plays a key part in various classical and quantum phenomena. Several experiments(2-4) have shown that in thin superconducting films, disorder enforces the droplet- like electronic texture - superconducting islands immersed into a normal matrix - and that tuning disorder drives the system from superconducting to insulating behaviour. In the vicinity of the transition, a distinct state(4) forms: a Cooper- pair insulator, with thermally activated conductivity. It results from synchronization of the phase of the superconducting order parameter at the islands across the whole system(5). Here we show that at a certain finite temperature, a Cooper- pair insulator undergoes a transition to a superinsulating state with infinite resistance. We present experimental evidence of this transition in titanium nitride films and show that the superinsulating state is dual to the superconducting state: it is destroyed by a sufficiently strong critical magnetic field, and breaks down at some critical voltage that is analogous to the critical current in superconductors.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.8
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Correction Chemistry, Applied

A detailed ellipsometric porosimetry and positron annihilation spectroscopy study of porous organosilicate-glass films with various ratios of methyl terminal and ethylene bridging groups (vol 306, 110434, 2020)

M. Rasadujjaman, Y. Wang, L. Zhang, S. Naumov, A. G. Attallah, M. O. Liedke, N. Koehler, M. Redzheb, A. S. Vishnevskiy, D. S. Seregin, Y. Wu, J. Zhang, J. Leu, A. Wagner, K. A. Vorotilov, S. E. Schulz, M. R. Baklanov

MICROPOROUS AND MESOPOROUS MATERIALS (2021)

Article Materials Science, Multidisciplinary

Charge Transport Mechanism and Trap Origin in Methyl-Terminated Organosilicate Glass Low-κ Dielectrics

Timofey V. Perevalov, Andrei A. Gismatulin, Andrei E. Dolbak, Vladimir A. Gritsenko, Elena S. Trofimova, Vladimir A. Pustovarov, Dmitry S. Seregin, Konstantin A. Vorotilov, Mikhail R. Baklanov

Summary: The study investigates the charge transport and trap nature responsible for the leakage current in thermally cured methyl-terminated organosilicate low-k dielectric films, revealing that the charge transport occurs via phonon-assisted electron tunneling between neutral traps. The obtained thermal trap energy value is close to that of oxygen divacancies, confirming the presence of oxygen vacancy and divacancy in the studied films. The Nasyrov-Gritsenko model accurately describes the charge transport mechanism, highlighting the importance of oxygen divacancies as traps for the leakage current.

PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE (2021)

Article Physics, Condensed Matter

Effect of Rashba and Dresselhaus spin-orbit coupling on supercurrent rectification and magnetochiral anisotropy of ballistic Josephson junctions

C. Baumgartner, L. Fuchs, A. Costa, Jordi Pico-Cortes, S. Reinhardt, S. Gronin, G. C. Gardner, T. Lindemann, M. J. Manfra, P. E. Faria Junior, D. Kochan, J. Fabian, N. Paradiso, C. Strunk

Summary: The simultaneous breaking of inversion- and time-reversal symmetry in Josephson junction (JJ) leads to anomalous Josephson effect and magnetochiral anisotropy (MCA) of Josephson inductance. The orientation of the current with respect to the lattice affects the MCA, possibly due to a finite Dresselhaus component, and the two-fold symmetry of the Josephson inductance reflects in the activation energy for phase slips.

JOURNAL OF PHYSICS-CONDENSED MATTER (2022)

Article Nanoscience & Nanotechnology

Supercurrent rectification and magnetochiral effects in symmetric Josephson junctions

Christian Baumgartner, Lorenz Fuchs, Andreas Costa, Simon Reinhardt, Sergei Gronin, Geoffrey C. Gardner, Tyler Lindemann, Michael J. Manfra, Paulo E. Faria Junior, Denis Kochan, Jaroslav Fabian, Nicola Paradiso, Christoph Strunk

Summary: This study introduces the design and application of non-reciprocal superconducting devices. By fabricating and measuring Josephson junctions, researchers have successfully achieved rectification of supercurrent and proposed a semi-quantitative model to explain the experimental data.

NATURE NANOTECHNOLOGY (2022)

Article Engineering, Electrical & Electronic

Charge Transport Mechanism in a PECVD Deposited Low-k SiOCH Dielectric

T. Perevalov, A. A. Gismatulin, V. A. Gritsenko, H. Xu, J. Zhang, K. A. Vorotilov, M. R. Baklanov

Summary: This study analyzes four bulk-limited models of charge transport and finds that phonon-assisted electron tunneling can explain the experimental results reasonably, with a thermal trap energy value of 1.2 eV. The trap nature is discussed, as well as a comparison with low-k films prepared using spin-on-glass technology.

JOURNAL OF ELECTRONIC MATERIALS (2022)

Article Physics, Applied

Effect of H atoms and UV wideband radiation on cured low-k OSG films

D. Lopaev, A. Zotovich, S. M. Zyryanov, M. A. Bogdanova, T. Rakhimova, Y. A. Mankelevich, N. N. Novikova, D. S. Seregin, A. S. Vishnevskiy, K. A. Vorotilov, Xiaoping Shi, M. R. Baklanov

Summary: The effects of hydrogen atoms and UV radiation on nanoporous organosilicate glass low-k films were studied. It was found that exposure to hydrogen atoms at low temperature caused slight modification of hydrocarbon bonds in hydrocarbon residues, while high temperature led to the destruction of Si-O and Si-CH2 groups. Additionally, the temperature increase also resulted in slight modification of the matrix structure. UV radiation had almost no effect on these processes.

JOURNAL OF PHYSICS D-APPLIED PHYSICS (2022)

Article Chemistry, Multidisciplinary

In-Situ Imaging of a Light-Induced Modification Process in Organo-Silica Films via Time-Domain Brillouin Scattering

Sathyan Sandeep, Alexey S. Vishnevskiy, Samuel Raetz, Sergej Naumov, Dmitry S. Seregin, Artem Husiev, Konstantin A. Vorotilov, Vitalyi E. Gusev, Mikhail R. Baklanov

Summary: The characterization of porogen-based organosilicate glass (OGS) films deposited by spin-on-glass technology was carried out using time-domain Brillouin scattering (TDBS). Remarkable differences between the films were revealed through the temporal evolution of the Brillouin frequency (BF) shift in TDBS experiments. The observed modification of the BF was correlated to the amount of carbon residue in the samples, the use of ultraviolet (UV) femtosecond probe laser pulses, and their intensity. The possibility of local modifications of OSG films with a nanometric resolution via nonlinear optical processes was demonstrated.

NANOMATERIALS (2022)

Article Materials Science, Multidisciplinary

Benzene bridged hybrid organosilicate films with improved stiffness and small pore size

A. A. Rezvanov, A. S. Vishnevskiy, D. S. Seregin, D. Schneider, A. A. Lomov, K. A. Vorotilov, M. R. Baklanov

Summary: The critical properties of porous periodic mesoporous silica low-k dielectric with different ratios of benzene bridges and methyl terminal groups were studied using advanced instrumentations such as Ellipso-metric Porosimetry, Surface Acoustic Wave Spectroscopy, and Specular X-ray reflectivity. The increase in benzene bridge concentration was found to decrease pore size and surface roughness, increase dielectric constant, and improve mechanical properties. Additionally, a percolation-type behavior of Young's modulus was observed with a sharp increase near a 50 mol % concentration of the benzene bridge.

MATERIALS CHEMISTRY AND PHYSICS (2022)

Article Physics, Applied

Damage to OSG low-k films during IPVD deposition of the Ta barrier layer

Alexander O. Serov, Alexey N. Ryabinkin, Alexey S. Vishnevskiy, Sergej Naumov, Alexander F. Pal, Tatyana V. Rakhimova, Dmitry S. Seregin, Konstantin A. Vorotilov, Mikhail R. Baklanov

Summary: The degradation of a porous organosilicate glass low-k dielectric during ionized physical vapor deposition of tantalum coating is mainly caused by vacuum UV flux from the argon inductively coupled plasma, not by direct current magnetron sputter plasma. The damage is associated with the removal of carbon-containing groups and breaking of Si-O bonds, resulting in the formation of hydrophilic Si-OH and Si-H groups. Therefore, the degree of damage can exceed expectations.

PLASMA PROCESSES AND POLYMERS (2023)

Article Chemistry, Multidisciplinary

UV-Excited Luminescence in Porous Organosilica Films with Various Organic Components

Md Rasadujjaman, Jinming Zhang, Dmitry A. Spassky, Sergej Naumov, Alexey S. Vishnevskiy, Konstantin A. Vorotilov, Jiang Yan, Jing Zhang, Mikhail R. Baklanov

Summary: The UV-induced photoluminescence of organosilica films with specific chemical groups was studied to understand the nature and origin of optically active defects. It was found that the sources of luminescence were carbon-containing components and carbon residues formed during the sample preparation process. A good correlation between the photoluminescence peaks and chemical composition was observed. The intensity of photoluminescence increased with porosity and internal surface area, and additional bands appeared after annealing, indicating changes in the matrix and segregation of residues on the surface.

NANOMATERIALS (2023)

Review Materials Science, Coatings & Films

Challenges in porosity characterization of thin films: Cross-evaluation of different techniques

Mikhail R. Baklanov, Konstantin P. Mogilnikov, Alexey S. Vishnevskiy

Summary: The review article provides an overview of important techniques for evaluating the porosity of thin films. These methods include ellipsometric porosimetry (EP), positron annihilation spectroscopy (PAS/PALS), and grazing incidence small-angle x-ray scattering (GISAXS). The article highlights the challenges and limitations of each method and demonstrates their unique insights into pore structure. The cross-evaluation of different methods enhances understanding of complex pore structures and emphasizes the importance of appropriate data modeling and interpretation.

JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A (2023)

Article Materials Science, Multidisciplinary

Structural and Luminescence Properties of Eu-Doped PMO Films with Ethylene Bridge and Methyl Terminal Groups

Md Rasadujjaman, Jinming Zhang, Alexey S. Vishnevskiy, Jing Zhang, Mikhail R. Baklanov

Summary: Eu-doped periodic mesoporous organosilicate (PMO) films have been successfully synthesized using sol-gel technology and spin-coating. The Eu doping alters the properties of the films and introduces luminescence emission. This study is significant for the development of novel functional organosilica materials.

COATINGS (2023)

Article Engineering, Electrical & Electronic

Modification of Porous Ultralow-k Film by Vacuum UltravioletEmission

Alexey Zotovich, Sergey M. Zyryanov, Dmitry Lopaev, Askar A. Rezvanov, Ahmed G. Attallah, Maciej O. Liedke, Maik Butterling, Maria A. Bogdanova, Alexey S. Vishnevskiy, Dmitry S. Seregin, Dmitry A. Vorotyntsev, Alexander P. Palov, Eric Hirschmann, Andreas Wagner, Sergej Naumov, Konstantin A. Vorotilov, Tatyana Rakhimova, Alexander T. Rakhimov, Mikhail R. Baklanov

Summary: This study investigates the modification of spin-on-deposited porous PMO ultralow-k SiCOH films by vacuum ultraviolet (VUV) emission. The results show that the VUV exposure process can be divided into two phases, with the first phase resulting in the removal of surface methyl and matrix bridging groups. This leads to increased material porosity. In the second phase, there is an increase in mesopore size, which is masked by air exposure.

ACS APPLIED ELECTRONIC MATERIALS (2022)

Article Physics, Multidisciplinary

4π-periodic supercurrent tuned by an axial magnetic flux in topological insulator nanowires

Ralf Fischer, Jordi Pico-Cortes, Wolfgang Himmler, Gloria Platero, Milena Grifoni, Dmitriy A. Kozlov, N. N. Mikhailov, Sergey A. Dvoretsky, Christoph Strunk, Dieter Weiss

Summary: This article investigates the topological transition in Josephson junctions based on topological insulator nanowires under different magnetic flux. The results show that the supercurrent is largely trivial at lower magnetic fields, but topological 4pi-periodic supercurrents start to appear at higher magnetic fields.

PHYSICAL REVIEW RESEARCH (2022)

Proceedings Paper Engineering, Electrical & Electronic

Mechanical Properties of Low-k Dielectric Deposited on Subtractively Patterned Cu Lines for Advanced Interconnects

I. S. Ovchinnikov, D. S. Seregin, D. A. Abdullaev, K. A. Vorotilov, A. A. Rezvanov, V. A. Gvozdev, T. Blomberg, A. A. Veselov, M. R. Baklanov

Summary: The mechanical properties of low-k dielectric films deposited on a surface with patterned metal lines were evaluated using atomic force microscopy in PeakForce quantitative mapping mode. The Young's modulus of completely cured low-k films was found to depend on the position in the structure, decreasing with reduction of intermetal gap. A significant reduction in Young's modulus was observed near the interface between the metal and low-k, possibly due to poor adhesion between the low-k film and barrier layers and a decrease in effective network connectivity of silicon atoms.

IITC2021: 2021 IEEE INTERNATIONAL INTERCONNECT TECHNOLOGY CONFERENCE (IITC) (2021)

暂无数据