Article
Physics, Multidisciplinary
S. Ghosh, J. R. Danielson, C. M. Surko
Summary: Measurements of positron annihilation as a function of energy in benzene reveal unexpected resonances, providing insights into the bonding nature of positron-molecule interactions and their relationship to the unique structure of benzene.
PHYSICAL REVIEW LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Elie Geagea, Judicael Jeannoutot, Michel Feron, Frank Palmino, Christophe M. Thomas, Alain Rochefort, Frederic Cherioux
Summary: Researchers have developed a new strategy to control the on-surface radical oligomerisations by using tunneling electrons, leading to the controlled synthesis of alkyl oligomers. This transfer only occurs under specific conditions, allowing for the precise formation of oligomers with defined size distribution.
Article
Physics, Applied
M. Faley, H. Fiadziushkin, B. Frohn, P. Schuffelgen, R. E. Dunin-Borkowski
Summary: This study reports the fabrication and characterization of titanium nitride nanobridge Josephson junctions and nanoscale superconducting quantum interference devices on SiN-buffered Si substrates. The use of titanium nitride allows for reproducible preparation and long-term stability of the devices. The variable thickness shape of the nanobridge junctions is achieved through wet etching and reactive ion etching. The results pave the way for superconducting electronics and all-TiN qubits operating at sub-100 mK temperatures.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2022)
Article
Physics, Applied
M. Faley, Timur Bikulov, Vincent Bosboom, A. A. Golubov, R. E. Dunin-Borkowski
Summary: Research has fabricated nanometer-scale superconducting quantum interference devices within a distance of 1 μm from the corners of 2 xx.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2021)
Article
Chemistry, Multidisciplinary
Michael Faley, Yuchen Liu, Rafal E. Dunin-Borkowski
Summary: The article describes nanobridge Josephson junctions and nanoSQUIDs based on TiN thin films, which exhibit high superconducting transition temperatures and coherence lengths. The fabricated nano-devices show stable characteristics, offering new prospects for superconducting electronics.
Article
Chemistry, Physical
Yuzhu Lu, Rulin Tang, Chuangang Ning
Summary: Sigma-type and pi-type excited dipole-bound states (DBSs) were observed in cryogenically cooled potassium iodide (KI) anions for the first time. Experimental and theoretical results showed excellent agreement, confirming the prediction that a dipolar molecule with a large enough dipole moment can have an excited DBS.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2021)
Article
Optics
Ryusei Iida, Haruya Suzuki, Toshiyuki Takayanagi, Masanori Tachikawa
Summary: In this study, positron-electron annihilation spectra of benzene, deuterated benzene, and naphthalene were theoretically calculated using Feshbach vibrational resonance energies and widths. It was found that the contribution of symmetric ring stretching vibration mode to the annihilation spectrum is significant and affects the p-electron density.
Article
Physics, Applied
Jorge Berger, Edson Sardella
Summary: The Keldysh-Usadel technique (KUT) is necessary for describing non-equilibrium situations in a superconductor below its critical temperature, but it has not been applied to realistic circuits. To check the validity of this procedure, a toy model (the Ginzburg-Landau model) is used in situations with slow evolution. It is found that neglecting the explicit influence of time variation leads to inaccurate or even qualitatively wrong description of phase slips.
PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS
(2022)
Article
Chemistry, Physical
Deb Kumar Bhowmick, Adrian Joe Urban, Manfred Bartsch, Bjoern Braunschweig, Helmut Zacharias
Summary: Efficient control of interface chemistry enables better tunability of electronic properties, and a novel near-UV-initiated direct modification method has been demonstrated to form stable organic monolayers on silicon surfaces with high hydrolytic stability.
JOURNAL OF PHYSICAL CHEMISTRY C
(2022)
Review
Chemistry, Inorganic & Nuclear
Guillem Gabarro-Riera, Guillem Aromi, E. Carolina Sanudo
Summary: This critical review covers the latest research on surface deposition of complex magnetic molecules, including deposition methods, surface types, and molecule characterization methods. Relevant examples are provided. Readers will gain an overview of the field and acquire tools to design their own experiments.
COORDINATION CHEMISTRY REVIEWS
(2023)
Article
Computer Science, Information Systems
M. Faley, R. E. Dunin-Borkowski
Summary: We have developed a self-biased planar 4-Josephson-junction nanoscale superconducting quantum interference device (nanoSQUID) with optimal sensitivity without the need for a magnetic flux. The nanoSQUID includes novel NbN-TiN-NbN nanobridge Josephson junctions (nJJs) with NbN current leads and TiN nanobridges connecting the electrodes of the nanoSQUID body. The nJJ and nanoSQUID exhibit hysteresis-free, reproducible, and long-term stable operation at 4.2 K, thanks to the optimal superconducting transition temperature and corrosion resistance of the TiN and NbN films. The nanoSQUID's cantilever is fabricated with a distance of approximately 300 nm between the nanoSQUID and the substrate corner, using amorphous Al films as sacrificial layers.
Article
Chemistry, Physical
Mengyuan Fan, Jingchen Xie, Xiao-Fei Gao, Bin Wu, Minfu Zhao, Shan Xi Tian
Summary: In this study, dissociative electron attachments of CO2- via the lowest shape resonant state (2)Pi(u) were investigated using a high-resolution anion velocity map imaging apparatus. The results showed that the dissociation of CO2-((2)Pi(u)) proceeds through a combinational motion of bond stretching and bending. This study provides important insights into the dissociation dynamics of CO2-((2)Pi(u)).
JOURNAL OF PHYSICAL CHEMISTRY A
(2022)
Article
Psychology, Multidisciplinary
Zhounan Huangfu, Lei Zhou, Jing Zhao, Sombat Kotchasit, Wanmei Chen
Summary: This study constructs a theoretical model to explore the mechanism of psychological needs on relationship quality in short video applications users. The results indicate that emotional attachment plays a positive role in relationship quality and attachment anxiety moderates the relationship between emotional attachment and relationship quality.
FRONTIERS IN PSYCHOLOGY
(2022)
Article
Multidisciplinary Sciences
Qing-Bin Lu
Summary: This paper proposes the cosmic ray-driven electron-induced reaction as a universal mechanism to quantitatively understand global ozone depletion. By deriving an analytical equation and comparing with observations, the results show that the equation can accurately describe ozone depletion globally. Additionally, the paper also discovers the impact of denitrification on ozone loss.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2023)
Article
Chemistry, Multidisciplinary
Trang Ngoc Huyen Bui, Yuriko Komagamine, Sahaprom Namano, Anna Miyayasu, Daisuke Sato, Shunsuke Minakuchi, Manabu Kanazawa
Summary: This study aimed to provide 5-year follow-up data comparing patient-reported outcomes for mandibular overdentures supported by two implants with magnetic attachments under immediate or conventional loading. Results showed no significant differences between the immediate loading group and the conventional loading group throughout the study. However, significant improvements in oral health-related quality of life, patient satisfaction, and denture assessment were observed within both groups from baseline to years 1-5.
APPLIED SCIENCES-BASEL
(2023)
Article
Physics, Applied
M. Ohkubo, G. Uehara, J. Beyer, M. Mimura, H. Tanaka, K. Ehara, S. Tanaka, T. Noguchi, E. E. Mitchell, C. P. Foley, R. L. Fagaly
Summary: This paper proposes a standard measurement method for determining R(n) and I(ci) in high-T(c) superconductors and low-T(c) multilayer superconductor/normal-conductor/superconductor (SNS) Josephson junctions, eliminating distortion effects on the U-I curves.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2022)
Article
Engineering, Electrical & Electronic
Simon K. H. Lam, Keith E. Leslie, Jeina Lazar
Summary: The article investigates the fabrication and optimization of Rf SQUIDs on MgO substrate. Ion beam etching as a post fabrication trimming process is used for noise optimization, but it degrades the low frequency 1/f noise. It is found that similar noise performance can be achieved in SQUIDs without the need of trimming.
IEEE TRANSACTIONS ON APPLIED SUPERCONDUCTIVITY
(2022)
Article
Nanoscience & Nanotechnology
Yichao Wang, Ali Zavabeti, Qifeng Yao, Thi Linh Chi Tran, Wenrong Yang, Lingxue Kong, David Cahill
Summary: Nanobionics-driven synthesis is an environmentally friendly approach for designing and synthesizing functional materials on a nanoscale. In this work, plasmonic HxMoO3 was synthesized using a green nanobionics approach by interacting chloroplasts with MoO3 nanoflakes. The synthesized plasmonic materials showed tunable plasmon resonances and high photocatalytic activities.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Chemistry, Multidisciplinary
Dulini Fernando, Motilal Mathesh, Jackie Cai, Wenrong Yang
Summary: A facile polymer-directed metal-organic framework (MOF)-based nanoarchitechtonics was developed to enhance the catalytic efficiency of multi-enzyme cascade reactions through substrate channeling. The new method involved the simultaneous synthesis of MOF and co-immobilization of enzymes, resulting in a closely packed nanoarchitecture with enhanced substrate channeling. The enzyme cascade reaction system showed a 3.5-fold increase in catalytic activity compared to free enzymes.
Article
Chemistry, Analytical
Yingqin Zhang, Ying Liao, Xuehu Yin, Yanli Zhang, Zhi Yang, Hongbin Wang, Wenrong Yang, Pengfei Pang
Summary: An electrochemical biosensor based on rolling circle amplification (RCA) was developed for the detection of lead ion (Pb2+). The biosensor utilized Pb2+-dependent DNAzyme and DNA-templated silver nanoclusters (DNA-AgNCs) for amplification, and showed high sensitivity and selectivity for Pb2+ analysis in the range of 1 pM-10 μM with a detection limit of 0.3 pM. This strategy has potential applications in real water samples and environment analysis.
MICROCHEMICAL JOURNAL
(2023)
Article
Chemistry, Multidisciplinary
Ru Feng, Hanqing Yin, Fuhao Jin, Wei Niu, Wanting Zhang, Jingquan Liu, Aijun Du, Wenrong Yang, Zhen Liu
Summary: This study demonstrates that NbB2 nanoflakes exhibit excellent selectivity and durability in ambient electrochemical N-2 reduction reaction, leading to efficient NH3 production. The high selectivity is attributed to the presence of abundant active vacancies on the surface, which makes the N-N triple bonds in N-2 molecule easier to break for NH3 production.
Article
Agriculture, Multidisciplinary
Nandini Bhattacharya, Mandira Kochar, Himadri B. Bohidar, Wenrong Yang, David M. Cahill
Summary: Reduced graphene oxide, bio-reduced using a microbial source, was used as a nanocarrier for the efficient delivery of the plant growth regulator, indole acetic acid, to maize plants. The loaded reduced graphene oxide displayed sustained release behavior and significantly enhanced the growth of maize plants.
ACS AGRICULTURAL SCIENCE & TECHNOLOGY
(2023)
Review
Agriculture, Multidisciplinary
Ananya Padmakumar, Chowdary Pavani, Kalyani Eswar, Lingxue Kong, Wenrong Yang, Subramanium Gopalakrishnan, David Miles Cahill, Aravind Kumar Rengan
Summary: The use of bacterial biocontrol agents (BBCAs) in plant protection has increased due to the rising awareness of chemical risks and the need for sustainable agriculture. Nanotechnology has facilitated the development of efficient and ecologically sound nanoformulations, such as bacteria premised nanobiopesticides (B-NBPs). These B-NBPs are synthesized using nanomaterials with amended properties at the nanoscale. This article provides an overview of BBCAs and their antagonistic mechanisms, focusing on the significance of BNPs in plant infection management and addressing concerns related to the efficacy of B-NBPs.
ACS AGRICULTURAL SCIENCE & TECHNOLOGY
(2023)
Article
Chemistry, Physical
Na Kong, Jin He, Wenrong Yang
Summary: Controlling and understanding the chemistry of molecular junctions is important in various fields. Stochastic single-entity collision electrochemistry (SECE) provides powerful tools to study single entities at the nanoscale. Molecular junctions formed by SECE collision have potential applications in monitoring molecular dynamics with high spatial and temporal resolution.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2023)
Article
Chemistry, Analytical
Yuru Min, Donglei Fu, Honglei Liu, Chenyao Yuan, Lei Wang, Mengyu Cao, Aowei Sun, Wenrong Yang, Jingquan Liu
Summary: Oxalyldihydrazide has been found to be an effective analytical reagent for determining formaldehyde and its analogs. By using UV-vis spectrophotometry, formaldehyde and other similar compounds like acetaldehyde, acetone, and benzaldehyde can be detected in solution. This method is also applicable for detecting formaldehyde in clams with high selectivity and sensitivity.
CHINESE JOURNAL OF ANALYTICAL CHEMISTRY
(2023)
Article
Chemistry, Multidisciplinary
Xiangyu Zhang, Kai Zhao, Hong Li, Yanhui Li, Wenrong Yang, Jingquan Liu, Da Li
Summary: Developing noble-metal-free bifunctional electrocatalysts with high catalytic ability at an effective cost for hydrogen production via water-splitting is crucial. The plasma engraving strategy is used to synthesize N-doped CoFeS on cobalt foam with a multi-interface and defect hierarchical structure.
NEW JOURNAL OF CHEMISTRY
(2023)
Article
Agriculture, Multidisciplinary
Anamika Pal, Pawan Kaur, Neeraj Dwivedi, Jim Rookes, Himadri B. Bohidar, Wenrong Yang, David Miles Cahill, Palash Kumar Manna
Summary: Clay-nanocomposite materials have been widely used for drug delivery systems, but their application in agriculture is less explored. The combination of nanoclay and active ingredients can create a biocompatible and environmentally friendly delivery vehicle for micronutrients, pesticides, etc., improving crop growth. This review provides an overview of the synthesis and application of clay-based nanocomposites in agriculture, addressing issues related to the delivery of active ingredients and biological macromolecules for crop protection and sustainability.
ACS AGRICULTURAL SCIENCE & TECHNOLOGY
(2023)
Article
Chemistry, Inorganic & Nuclear
Xiangyu Zhang, Hong Li, Yanhui Li, Xianhui Wang, Hongbin Wang, Wenrong Yang, Jingquan Liu, Da Li
Summary: To replace expensive precious metal catalysts, it is important to develop inexpensive and powerful bifunctional catalysts for hydrogen production. In this study, a hierarchical structure Fe-Co3S4/MoS2 catalyst was synthesized using excellent templates and elemental doping, demonstrating excellent catalytic performance and long-term stability for overall water splitting.
DALTON TRANSACTIONS
(2023)
Article
Chemistry, Inorganic & Nuclear
Xiangyu Zhang, Hong Li, Yanhui Li, Xianhui Wang, Hongbin Wang, Wenrong Yang, Jingquan Liu, Da Li
Summary: To replace expensive precious metal catalysts for water electrolysis, it is important to develop inexpensive and powerful bifunctional catalysts. In this study, a hierarchical structure Fe-Co3S4/MoS2 catalyst was synthesized and showed excellent catalytic performance and stability for overall water splitting. The Fe doping and component modulation contributed to the high intrinsic activity and excellent transfer coefficients of the catalyst.
DALTON TRANSACTIONS
(2023)
Article
Materials Science, Multidisciplinary
Andrew D. Squires, Xiang Gao, Jia Du, Zhaojun Han, Dong Han Seo, James S. Cooper, Adrian T. Murdock, Simon K. H. Lam, Ting Zhang, Tim van der Laan
Summary: This research proposes a graphene/gold bilayer metasurface as a reconfigurable and tunable material for terahertz electronic devices. A frequency-selective absorber with electrical tuning in the 0.1-1 THz range is created using this material. This study is crucial for the development of high-speed wireless communication and sensing technologies.
COMMUNICATIONS MATERIALS
(2022)