期刊
RADIOCHIMICA ACTA
卷 103, 期 3, 页码 205-211出版社
WALTER DE GRUYTER GMBH
DOI: 10.1515/ract-2014-2336
关键词
Actinide; Sorption; Nanodiamond
资金
- Russian Science Foundation [14-13-01279]
- Russian Foundation for Basic Research [12-05-00208]
- M.V. Lomonosov Moscow State University Program of Development
- Russian Science Foundation [14-13-01279] Funding Source: Russian Science Foundation
Detonation nanodiamonds (ND) present a significant part of nanocarbons group, which could be produced on commercial scale by detonation of explosives in a closed chamber. Their unique properties of high surface area, low weight and radiation resistance make ND a prospective candidate for applications in sorption processes in radiochemistry. To study the influence of surface chemistry on sorption properties, apristine sample of ND was treated with acids and hydrogen. The surface chemistry of the samples was characterised by infrared spectroscopy, X-ray photoelectron spectroscopy and Boehm titration. The sorption properties of ND were tested fordifferent radionuclides. The sorption capacity of ND was shown to be higher than those of commonly used radionuclide sorbents like activated carbon and compariable to other members of nanocarbon group like graphene oxide and carbon nanotubes. The sorption properties were shown to be influenced by the presence of oxygen-containing groups on the surface of ND. This represents an opportunity to increase the sorption capacity of ND.
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