Article
Multidisciplinary Sciences
Carolina A. Marques, Luke C. Rhodes, Izidor Benedicic, Masahiro Naritsuka, Aaron B. Naden, Zhiwei Li, Alexander C. Komarek, Andrew P. Mackenzie, Peter Wahl
Summary: The phenomenon and radical changes observed in material properties during a quantum phase transition have attracted significant attention in condensed matter research in recent decades. Strong electronic correlations give rise to exotic electronic ground states, such as magnetic order, nematicity, and unconventional superconductivity. A detailed understanding of the electronic structure near the Fermi energy is necessary to provide a microscopic model for these phenomena and achieve a complete understanding of the physics of the quantum critical point.
Article
Physics, Particles & Fields
Guruprasad Kadam, Hiranmaya Mishra, Marco Panero
Summary: In this study, we found that the shear viscosity to entropy density ratio decreases and the bulk viscosity coefficient rises rapidly near the QCD critical point.
EUROPEAN PHYSICAL JOURNAL C
(2021)
Article
Materials Science, Multidisciplinary
Zhentao Wang, Dominique Gautreau, Turan Birol, Rafael M. Fernandes
Summary: Rare-earth titanates are Mott insulators whose magnetic ground state can be tuned between antiferromagnetic and ferromagnetic states by substituting rare-earth elements. This study combines phenomenology and first-principles calculations to analyze the magnetic phase diagram and reveals the presence of a first-order metamagnetic transition line and a Widom line that can be tuned to zero temperature using strain.
Article
Multidisciplinary Sciences
An Wang, Feng Du, Yongjun Zhang, David Graf, Bin Shen, Ye Chen, Yang Liu, Michael Smidman, Chao Cao, Frank Steglich, Huiqiu Yuan
Summary: Ferromagnetic quantum criticality was observed in CeRh6Ge4 under moderate hydrostatic pressure, supported by quantum oscillation measurements. The study found that Ce 4f electrons remain localized and do not contribute to the Fermi surface, suggesting localized ferromagnetism as a key factor for the occurrence of a ferromagnetic quantum critical point in CeRh6Ge4.
Article
Physics, Multidisciplinary
Hiroyuki Yamase
Summary: We have conducted a microscopic study on itinerant ferromagnetic systems and discovered a highly diverse phase diagram in the three-dimensional space of chemical potential, magnetic field, and temperature. This extends beyond the Landau theory that has been analyzed so far. In addition to the generic wing structure near the tricritical point when introducing a magnetic field, we also observed the generation of an additional wing near a quantum critical end point (QCEP) and even from within the ferromagnetic phase. The tilting of the wing controls the entropy jump associated with the metamagnetic transition.
NEW JOURNAL OF PHYSICS
(2023)
Article
Astronomy & Astrophysics
Julian Bernhardt, Christian S. Fischer, Philipp Isserstedt, Bernd-Jochen Schaefer
Summary: This study investigates the impact of finite volume and the corresponding restrictions on long-range correlations on the location of the critical endpoint in the QCD phase diagram. Utilizing a combination of lattice Yang-Mills theory and truncated versions of Dyson-Schwingcr equations, the researchers found that the critical endpoint's location is dependent on volume and boundary conditions. Notable volume effects are observed for volumes less than or equal to 5 fm, with larger volumes approaching the infinite-volume limit.
Article
Astronomy & Astrophysics
Peter Kovacs, Gyozo Kovacs, Francesco Giacosa
Summary: The phase diagram of quantum chromodynamics (QCD) was investigated by varying the number of colors Nc within a Polyakov loop quark-meson chiral model. The results showed that the critical point(s) changed their positions and characteristics with different numbers of colors, and a distinct symmetry was observed in the phase diagram at large Nc.
Article
Nanoscience & Nanotechnology
Sabyasachi Tiwari, Maarten L. Van de Put, Bart Soree, William G. Vandenberghe
Summary: Using first-principles calculations, the magnetic order in 2D TMD monolayers doped with transition metals was investigated, revealing five distinct magnetically ordered states among 35 TMD-dopant pairs. Different dopants result in different magnetic states, with Ni and Ti leading to non-magnetic states, Cr leading to antiferromagnetic states, and Fe, Mn, Co, and V leading to ferromagnetic states for most TMDs except MoTe2. V-doped MoSe2 and WSe2, and Mn-doped MoS2 were identified as the most suitable candidates for achieving room-temperature ferromagnetism at 16-18% atomic substitution.
NPJ 2D MATERIALS AND APPLICATIONS
(2021)
Article
Chemistry, Multidisciplinary
I. Benabdallah, A. Sibari, H. El Masaoudi, W. Azouzi, M. Benaissa
Summary: The present study extensively investigates the quantum confinement effect in phosphorene and black phosphorus quantum dots from both experimental and theoretical perspectives. The quantum structures were prepared using Liquid Phase Exfoliation and solvothermal-assisted Liquid Phase Exfoliation techniques. The results show that there is no phosphorus oxidation in both phosphorene and black phosphorus quantum dots solutions. Additionally, the Raman spectroscopy indicates a shift in B-2g and A(g)(2) phonon modes for phosphorene and black phosphorus quantum dots compared to bulk black phosphorus. The structural characterization reveals a high degree of crystallinity in both quantum structures with no sign of aggregations. The optical properties characterization confirms an expected increase in the bandgap value for both structures, which agrees with theoretical calculations. Interestingly, it is demonstrated that the quantum confinement observed in phosphorene is weakened to the expected extent, relative to that in BPQDs, by the loss of two confinement dimensions.
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
(2022)
Article
Astronomy & Astrophysics
Pascal J. Gunkel, Christian S. Fischer
Summary: By studying the effects of pion and sigma meson backcoupling on the chiral order parameters, we found a small shift of the critical endpoint towards smaller chemical potentials and a decrease in the curvature of the chiral crossover line. Our results suggest that the location of the critical endpoint in the phase diagram is mainly determined by the microscopic degrees of freedom of QCD.
Article
Physics, Multidisciplinary
Shaolong Zeng, Sue Ping Szeto, Fan Zhong
Summary: Phase transitions and critical phenomena are fascinating phenomena in nature, and the renormalization-group theory is a great achievement in theoretical physics for describing them. However, the theory fails to accurately predict above a critical dimension, leading to a discrepancy with reality. In this study, we offer a different perspective on the problem and reveal the origin of the inconsistencies in the existing scenarios. We also develop an effective-dimension theory that can account for all the existing results and predict new scaling behaviors.
Article
Physics, Fluids & Plasmas
Bruno Murta, J. Fernandez-Rossier
Summary: This article introduces Quintanilla's theorem, which establishes a one-to-one relation between zero-temperature static spin-spin correlators and coupling constants for quantum spin Hamiltonians. The theorem provides a theoretical foundation for learning quantum spin Hamiltonians using spin structure factors as input data. The validity of the theorem is extended to the case of finite-temperature spin structure factors, and it also applies to all types of Hamiltonians expressed as sums of bilinear operators.
Article
Chemistry, Inorganic & Nuclear
Nesrine Benamara, Zouaoui Setifi, Chen- Yang, Sylvain Bernes, David K. Geiger, Gunes Suheyla Kurkcuoglu, Fatima Setifi, Jan Reedijk
Summary: Two new compounds with general formula [M(N-3)(2)(dmbpy)], where dmbpy = 5,5'-dimethyl-2,2'-bipyridine and M = Mn(II) or Co(II), have been synthesized and characterized structurally and magnetically. Both compounds exhibit weak interchain interactions due to pi-pi stacking between the dmbpy rings. The manganese compound shows spin-canted antiferromagnetic ordering with metamagnetism, while the cobalt compound displays weak ferromagnetism and long-range magnetic ordering.
Article
Materials Science, Multidisciplinary
Giovanni Annur Safarina, Yong-Jin Kim, Chan -Ho Yang
Summary: We investigated the presence of cooperative Jahn-Teller distortion in LaMnO3 films grown on GdScO3 substrates using Raman spectroscopy. We observed a characteristic B1g phonon mode with preserved symmetry down to a two-unit-cell thickness, suggesting that there is no critical transition of the cooperative Jahn-Teller distortion and corresponding orbital order driven by film thickness when the two-dimensional distortion plane is parallel to the substrate.
Article
Materials Science, Multidisciplinary
Ming Xie, Sankar Das Sarma
Summary: The recent experimental discovery of flavor symmetry breaking metallic phases in Bernal-stacked bilayer graphene indicates the strong interaction between electrons near the top (bottom) of its valence (conduction) band. Superconductivity is observed in between these symmetry breaking phases when the graphene bilayer is subjected to a small in-plane magnetic field or is in close proximity to a monolayer WSe2 substrate. This study investigates the correlated nature of band edge electrons, obtaining the quantum phase diagram of their many-body ground states by considering the impact of proximity-induced spin-orbit coupling.
Article
Physics, Multidisciplinary
Jackson R. Badger, Yundi Quan, Matthew C. Staab, Shuntaro Sumita, Antonio Rossi, Kasey P. Devlin, Kelly Neubauer, Daniel S. Shulman, James C. Fettinger, Peter Klavins, Susan M. Kauzlarich, Dai Aoki, Inna M. Vishik, Warren E. Pickett, Valentin Taufour
Summary: Unconventional superconductors have Cooper pairs with lower symmetries compared to conventional superconductors. This article demonstrates that the time-reversal symmetry breaking in the superconductor LaNiGa2 is enabled by its previously unknown topological electronic band structure. These unique topological features allow LaNiGa2 to break time-reversal symmetry in the absence of other typical ingredients, providing a pathway for identifying a new type of unconventional superconductors based on nonsymmorphic symmetries.
COMMUNICATIONS PHYSICS
(2022)
Review
Physics, Condensed Matter
D. Aoki, J-P Brison, J. Flouquet, K. Ishida, G. Knebel, Y. Tokunaga, Y. Yanase
Summary: This article reviews the recent experimental and theoretical progress on the novel spin-triplet superconductor UTe2 and discusses its rich phase diagrams, unconventional behaviors, and the interplay between its normal and superconducting properties in different conditions.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2022)
Article
Physics, Condensed Matter
Zihao Shen, X. D. Zhu, Rahim R. Ullah, Peter Klavins, Valentin Taufour
Summary: In this study, we present the results of bulk magnetization measurements and spatially resolved measurements of magnetic domains in Co3Sn2S2.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2023)
Article
Chemistry, Inorganic & Nuclear
Ashlee K. Hauble, Kamil Ciesielski, Valentin Taufour, Eric S. Toberer, Susan M. Kauzlarich
Summary: In this study, Ba2-xEuxZnSb2 was synthesized by substituting Eu for Ba to improve the stability of the material in air and to characterize its thermal and electronic properties. The samples exhibited low thermal conductivity (<0.8 W/m K), high Seebeck coefficient (350-550 mu V/K), and high charge carrier mobility (20-35 cm2/V) from 300 to 500 K, consistent with predictions of high thermoelectric efficiency. Evaluation of the thermoelectric quality factor suggests that a higher zT can be achieved by increasing the carrier concentration through doping.
INORGANIC CHEMISTRY
(2023)
Editorial Material
Physics, Multidisciplinary
Dai Aoki, Ilya Sheikin, Alix McCollam, Jun Ishizuka, Youichi Yanase, Gerard Lapertot, Jacques Flouquet, Georg Knebel
Summary: In this study, de Haas -van Alphen (dHvA) experiments were performed in the spintriplet superconductor UTe2, revealing the presence of three fundamental dHvA frequencies and suggesting the existence of cylindrical Fermi surfaces. The possibility of small pocket Fermi surfaces associated with extremely heavy masses cannot be fully excluded.
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN
(2023)
Article
Physics, Multidisciplinary
Arvind Maurya, Hisatomo Harima, Fuminori Honda, Yusei Shimizu, Yoshiki J. Sato, Ai Nakamura, Dexin Li, Yoshiya Homma, Dai Aoki
Summary: In this study, we observed bulk superconductivity in LaNiZn below Tc = 1.5 K, as confirmed by its electrical transport and specific heat capacity (Delta Cel/gamma Tc = 1.41). The upper critical fields along the hexagonal crystallographic c-axis and in the basal plane at 30 mK were found to be 0.36 and 0.24 T, respectively, suggesting mainly an orbital mechanism for field-induced depairing and a negligible spin triplet component in the superconducting order parameter. The angular dependence of Hc2 is explained by an effective mass model with an oblate-shaped effective Fermi surface. Our experimental and band calculation under local density approximation results suggested that LaNiZn is a Bardeen- Cooper-Schrieffer s-wave-type superconductor in the dirty limit, possibly involving multiple bands.
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN
(2023)
Article
Multidisciplinary Sciences
Edwin Herrera, Isabel Guillamon, Victor Barrena, William J. Herrera, Jose Augusto Galvis, Alfredo Levy Yeyati, Jan Rusz, Peter M. Oppeneer, Georg Knebel, Jean Pascal Brison, Jacques Flouquet, Dai Aoki, Hermann Suderow
Summary: Two-dimensional electronic states are often observed at surfaces of wide-band metals, resulting from confinement by nanoscale closed geometries. In this study, we used scanning tunnelling microscopy to investigate atomically flat terraces on the surfaces of a heavy-fermion superconductor, URu2Si2. We observed two-dimensional heavy fermions with quantized energy levels separated by a fraction of a millielectronvolt, suggesting a new route to studying quantum-well states in strongly correlated quantum materials.
Article
Physics, Multidisciplinary
A. Rosuel, C. Marcenat, G. Knebel, T. Klein, A. Pourret, N. Marquardt, Q. Niu, S. Rousseau, A. Demuer, G. Seyfarth, G. Lapertot, D. Aoki, D. Braithwaite, J. Flouquet, J. P. Brison
Summary: The recently discovered superconductor UTe2, with a superconducting transition temperature Tc between 1.5 and 2 K, has raised great attention due to its strong suspicion of spin-triplet and topological superconductivity. The properties of UTe2 under a magnetic field are also remarkable, showing field-reinforced and field-induced superconducting phases. This study provides the first complete thermodynamic determination of the phase diagram for fields applied along different crystallographic directions, revealing a strong negative curvature of the upper critical field along the easy axis and the existence of a phase transition line within the superconducting phase.
Article
Physics, Multidisciplinary
Fabrice Wilhelm, Jean-Pierre Sanchez, Daniel Braithwaite, Georg Knebel, Gerard Lapertot, Andrei Rogalev
Summary: This article investigates the electronic structure of UTe2 through two types of X-ray spectroscopy, revealing unusual features and pressure dependence of the 5f electron count. This understanding is crucial for fully comprehending its superconducting properties.
COMMUNICATIONS PHYSICS
(2023)
Article
Physics, Applied
Joshua F. Belot, Valentin Taufour, Stefano Sanvito, Gus L. W. Hart
Summary: Researchers developed machine-learning models based on the chemical composition of materials to predict Curie temperatures. A random-forest model provided the most accurate predictions and did not require dimensionality reduction or complex descriptors. Cobalt-rich and iron-rich materials showed the highest Curie temperatures among binary and ternary compounds.
APPLIED PHYSICS LETTERS
(2023)
Article
Materials Science, Multidisciplinary
R. R. Ullah, P. Klavins, X. D. Zhu, V. Taufour
Summary: Two ferromagnetic phases, FM1 and FM2, were found to exist in LaCrGe3, and the domain structure undergoes a substantial change between these two phases. The measurements of the coercive field and magnetization curves reveal unconventional magnetic domain behavior in the FM1 phase, followed by a depinning region as the system transitions into the FM2 phase.
Article
Materials Science, Multidisciplinary
Arvind Maurya, Atsushi Miyake, Hisashi Kotegawa, Yusei Shimizu, Yoshiki J. Sato, Ai Nakamura, Dexin Li, Yoshiya Homma, Fuminori Honda, Masashi Tokunaga, Dai Aoki
Summary: We report the single-crystal growth of UNi4P2 and demonstrate its Ising-type ferromagnetism with a Curie temperature of 25 K through magnetization, electrical transport, and specific heat measurements. The strong anisotropy between the c axis and the tetragonal basal plane is maintained up to 57 T, while the intraplane anisotropy gradually disappears at higher fields. Our findings suggest that anisotropic electron correlations may stabilize Ising-type ferromagnetic order in one dimension at nonzero temperatures, potentially with its own characteristic universality class.
Article
Chemistry, Physical
Luke M. McClintock, Long Yuan, Ziyi Song, Michael T. Pettes, Dmitry Yarotski, Rijan Karkee, David A. Strubbe, Liang Z. Tan, Azza Ben-Akacha, Biwu Ma, Yunshu Shi, Valentin Taufour, Dong Yu
Summary: 1D organic metal halide hybrids (OMHHs) exhibit promising optical properties for photodetection and lighting applications, but the governing mechanisms and surface effects are not well understood. This study investigates the optical properties of 1D C4N2H14PbBr4 through polarization-dependent time-averaged and time-resolved photoluminescence spectroscopy. The results reveal an excitation-energy-dependent anisotropic emission, which is attributed to fast surface recombination confirmed by first-principles calculations and experimental measurements.
Article
Materials Science, Multidisciplinary
K. Kinjo, H. Fujibayashi, S. Kitagawa, K. Ishida, Y. Tokunaga, H. Sakai, S. Kambe, A. Nakamura, Y. Shimizu, Y. Homma, D. X. Li, F. Honda, D. Aoki, K. Hiraki, M. Kimata, T. Sasaki
Summary: UTe2 is a recently discovered spin-triplet superconductor with a magnetic field (H)-boosted superconductivity >16 T when H is applied exactly parallel to the b axis. The high-H superconducting (HHSC) phase of UTe2 has not been thoroughly investigated, and its SC properties as well as the spin state are not well understood. In this study, AC magnetic susceptibility and nuclear magnetic resonance measurements were performed, revealing that the HHSC state has bulk nature and is sensitive to the H angle, with different SC character compared to the low-H superconducting (LHSC) state. The dominant spin component of the spin-triplet pair also changes from the LHSC state (along the a axis) to the HHSC state (along the b axis). Our findings suggest that the H-induced multiple SC states originate from the remaining spin degrees of freedom.