期刊
POLYMER
卷 64, 期 -, 页码 62-68出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.polymer.2015.03.036
关键词
Tribology; Graphene; In-situ polymerization
资金
- National Natural Science Foundation of China (NSFC) [U1304212]
- Development Foundation for Distinguished Junior Researchers at Zhengzhou University [1421320043]
Graphene-oxide-hybrided polyurethane/epoxy interpenetrating polymer networks (PU/EP IPNs) are prepared through an in-situ polymerization. The results showed that the mechanical performance of graphene-oxide-hybrided PU/EP IPNs is improved due to the formation of chemical bonds between graphene oxide nanosheet and polyurethane/epoxy segments, affording the loading transfer from polymer matrix to graphene oxide nanosheet The average friction coefficient in the steady stage is decreased about 30.2% from neat PU/EP IPN to graphene-oxide-hybrided PU/EP IPNs. Especially, the specific wear rate is decreased about two orders of magnitude from neat PU/EP IPN to graphene-oxide-hybrided PU/EP IPNs. Interestingly, graphene-oxide-hybrided PU/EP IPNs have the same friction coefficient in the steady stage, independent of graphene oxide content. The identical steady friction coefficients are derived from the same friction bodies in three-body friction model, such as grapheneoxide-strengthened PU/EP IPN surface, metallic counterpart and graphene-oxide-wrapping polymer particles as wear debris in the transfer film. (C) 2015 Elsevier Ltd. All rights reserved.
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