期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 136, 期 49, 页码 17013-17015出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja511534x
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资金
- European Research Council [267281]
- EPSRC [EP/K039946/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K039946/1] Funding Source: researchfish
- European Research Council (ERC) [267281] Funding Source: European Research Council (ERC)
The total synthesis of hongoquercin B was carried out in 9 steps from trans,trans-farnesyl acetate using a palladium catalyzed decarboxylative pi-farnesyl rearrangement of a diketo-dioxinone ester, aromatization and cationic diene-epoxide cyclization as key steps. This cascade tetracyclization simplifies the synthesis of terpenoid resorcylate natural products.
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