期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 42, 页码 17354-17357出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja305991k
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资金
- Bristol-Myers Squibb
- Zhejiang University
- Hertz Foundation
- Harvard Undergraduate Research Program
A detailed stereomechanistic analysis has led to the design of a new tetradentate ligand for the enantioselective Ti(IV)-catalyzed oxidation of unsymmetrical sulfides to sulfoxides with high selectivity. The pathway of this oxidation and the closely related and long-known Kagan-Modena oxidation have been clarified to identify the likely origin of the enantioselectivity.
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