期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 134, 期 2, 页码 824-827出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja209729h
关键词
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资金
- National Natural Science Foundation of China [21002057, 21132005, 91127006, 21121004]
- National Basic Research Program of China (973 program) [2011CB932501]
- Tsinghua University Initiative
We report herein the synthesis of a new metal cluster-encapsulated supramolecular capsule, [(C C)@Ag5-6@(Py6)(2)](CF3SO3)(3-4)(3, Py6 = azacalix[6]-pyridine), by use of a bowl-shaped macrocyclic ligand Py6. The multinuclear silver carbide cluster aggregate in 3 is encapsulated by two Py6 ligands through both metal-ligand coordination and cation-pi interactions, spotlighting a new synthetic strategy for supramolecular capsules.
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