期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 132, 期 21, 页码 7246-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja101040s
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资金
- Grants-in-Aid for Scientific Research [20108006, 22245006] Funding Source: KAKEN
- Ministry of Education, Science & Technology (MoST), Republic of Korea [R32-2008-000-10217-0] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [R16-1997-011-01001-0, 2005-0093839] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
A meso,meso-diketohexaphyrin was isolated and characterized as a chemically stable non-Kekule singlet biradicaloid. Two unpaired electrons are seemingly delocalized on two tripyrrolic units separated by C=O bonds. These results underscore the potential of expanded porphyrins to achieve unique electronic states.
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