期刊
JOURNAL OF POWER SOURCES
卷 245, 期 -, 页码 958-966出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2013.07.054
关键词
Solid oxide fuel cells (SOFCs); Ceramic/glass seals; Binder burnout; Compression loading; Thermally-induced dimensional response
资金
- Ohio Department of Development's Third Frontier Fuel Cell Program
Solid oxide fuel cells (SOFCs) require seals that can function in harsh, elevated temperature environments. Comprehensive characterization and understanding of seals is needed for commercially viable SOFCs. The present research focuses on a novel ceramic/glass composite seal that is produced by roller compaction or tape casting of glass and ceramic powders and an organic binder. Upon heat treatment, micro-voids and surface anomalies are formed. Increased heating and cooling rates during the heat treatment resulted in more and larger voids. The first goal of the current research is to suggest an appropriate heating and cooling rate to minimize the formation of microstructural defects. After identifying an appropriate cure cycle, seals were thermally cycled and then characterized with laser dilatometry, X-ray diffraction, and sonic resonance. From these experiments the crystalline phases, thermal expansion, and elastic properties were determined. Subsequently compression testing with an acoustic emission (AE) sensor and post-test microstructural analysis were used to identify the formation of damage. By fully understanding the characteristics of this ceramic/glass composite seal, next generation seals can be fabricated for improved performance. (C) 2013 Elsevier B.V. All rights reserved.
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