期刊
JOURNAL OF POWER SOURCES
卷 243, 期 -, 页码 172-180出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2013.05.174
关键词
Solid oxide fuel cell (SOFC); Nickel-yttria stabilized zirconia (Ni-YSZ); Suspension plasma spraying (SPS); Axial injection
资金
- Natural Sciences and Engineering Research Council (NSERC) of Canada
- Solid Oxide Fuel Cells Canada Strategic Research Network
- NSERC
Composite Ni-Y0.15Zr0.85O1.925 anodes were fabricated by axial-injection suspension plasma spraying in open atmosphere conditions. The composition of the anode is controllable by adjustment of the plasma gas composition, stand-off distance, and suspension feed rate. The total porosity is controllable through the addition of carbon black to the suspension as a sacrificial pore-forming material as well as by adjustment of the suspension feed rate. The size of the NiO particles in suspension affects both the composition and total porosity, with larger NiO particles leading to increased Ni content and porosity in the deposited coatings. The surface roughness increases with a decrease of the in-flight droplet momentum, which results from both smaller NiO particles in suspension and the addition of low density pore-forming materials. A solid oxide fuel cell was fabricated with both electrodes and electrolyte fabricated by axial-injection plasma spraying. Peak power densities of 0.718 W cm(-2) and 1.13 W cm(-2) at 750 degrees C and 850 degrees C, respectively, were achieved. (C) 2013 Elsevier B.V. All rights reserved.
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