期刊
JOURNAL OF POWER SOURCES
卷 193, 期 1, 页码 367-370出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2008.11.106
关键词
Palladium; Polyelectrolyte; Polyacrylic acid; Hybrid nanoparticle; Hydrogen sensor
资金
- New Energy and Industrial Technology Development Organization (NEDO) of Japan
- Ministry of Education, Science, Sports, and Culture of Japan
We prepared palladium-polyelectrolyte hybrid nanoparticles by using a metallization of polyelectrolyte. In this study, we selected polyacrylic acid (PAA) as a polyelectrolyte and reduced the palladium ions on the PAA by using ascorbic acids in order to form a unique spherically shaped mosslike hybrid nanoparticle. Palladium (Pd) can absorb hydrogen to become PdHx, and the storage of hydrogen increases the electrical resistance and volume of Pd materials. The use of this material is attracting growing interest as a reliable, cheap, ultracompact, and safe hydrogen sensor for use in fuel cells. We showed the utilization of the Pd-PAA hybrid nanoparticles as a highly sensitive hydrogen sensor that exhibited a switch response depending on volume expansion in a cyclic atmosphere exchange. (C) 2008 Elsevier B.V. All rights reserved.
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