Article
Multidisciplinary Sciences
Zeyu Hao, A. M. Zimmerman, Patrick Ledwith, Eslam Khalaf, Danial Haie Najafabadi, Kenji Watanabe, Takashi Taniguchi, Ashvin Vishwanath, Philip Kim
Summary: By constructing a van der Waals heterostructure with three stacked graphene layers at alternating twist angles, researchers observed tunable superconductivity at a specific twist angle. The superconducting regions are associated with flavor polarization of moire bands and are bounded by a van Hove singularity at high displacement fields, indicating unconventional moire superconductivity.
Article
Chemistry, Multidisciplinary
Nikita Tepliakov, QuanSheng Wu, Oleg Yazyev
Summary: In this study, the intrinsic polarization and screening of multilayer graphene under an external electric field were investigated using density functional theory and the Wannier function formalism. It was found that multilayer graphene is intrinsically polarized due to the crystal field effect, which is often overlooked in tight-binding models. Different out-of-plane alignments were observed in ordered and twisted graphene multilayers, with a much stronger in-plane potential modulation in the twisted systems. Our findings provide insights into intrinsic and extrinsic polarization in graphene multilayers and offer parameters necessary for accurate modeling of these systems.
Article
Multidisciplinary Sciences
Haoxin Zhou, Ludwig Holleis, Yu Saito, Liam Cohen, William Huynh, Caitlin L. Patterson, Fangyuan Yang, Takashi Taniguchi, Kenji Watanabe, Andrea F. Young
Summary: Spin-polarized superconductivity is observed in Bernal bilayer graphene under a large applied perpendicular electric field. Electrostatic gate tuning leads to transitions between electronic phases with different polarizations in the spin space. A transition to a superconducting state is observed at a finite magnetic field, and the critical temperature is consistent with a spin-triplet order parameter.
Article
Chemistry, Physical
Bowen Shi, Haotian Wang, Wen Jiang, Yuan Feng, Pan Guo, Heng Gao, Zhibin Gao, Wei Ren
Summary: In this study, the physical properties of a heterobilayer composed of 2D graphene and hexagonal boron nitride (h-BN) are investigated using first-principles calculations and simulations. The binding energies, electric dipoles, and twisting angles of three stacking orders in the graphene/h-BN heterobilayer are calculated. It is found that the AB stacking structure exhibits the lowest energy. Furthermore, the electric field perpendicular to the 2D plane is found to control the dipole magnitude and polarization direction of the bilayer system. The kinetic and thermodynamic stability of graphene/h-BN heterobilayers under external electric fields are studied using Ab initio molecular dynamics (AIMD). The potential importance of graphene/h-BN heterobilayers in the field of information electronics is also proposed.
APPLIED SURFACE SCIENCE
(2023)
Article
Materials Science, Ceramics
Shuibao Liang, Xin-Ping Zhang
Summary: This study develops a phase field model to investigate grain-boundary (GB) migration in alumina (Al2O3). The results show that the electric field can enhance or inhibit GB migration, with the direction and strength of the field influencing the migration velocity and direction. The study reveals the competitive effect between curvature and electric field driving forces and derives an analytical expression for the critical electric field.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2023)
Article
Chemistry, Physical
Xian Wang, Yingqi Cui, Li Zhang, Mingli Yang
Summary: The study investigates the band gap variations of bilayer graphene quantum dots under the influence of external electric field and interlayer twist using a quantum-dot model and first-principles calculations. It is found that interlayer twist widens the gaps while applied field narrows them, with their coupling resulting in enhanced Stark response in twisted structures. This exceptional Stark shift is attributed to asynchronous shifts in occupied and virtual energy levels induced by the field, further enhanced by strong interlayer coupling at specific twist angles.
Article
Chemistry, Physical
Shuai Zhang, Qiang Xu, Yuan Hou, Aisheng Song, Yuan Ma, Lei Gao, Mengzhen Zhu, Tianbao Ma, Luqi Liu, Xi-Qiao Feng, Qunyang Li
Summary: In this study, two metastable reconstruction states with distinct stacking orders and strain soliton structures were identified in small-angle twisted graphene using conductive atomic force microscopy. The switching mechanism between these two states was found to propagate spontaneously in a domino-like fashion. The fine structure of the bistable states is critical for understanding the unique properties of van der Waals structures with tiny twists.
Article
Physics, Multidisciplinary
A. Schmitt, P. Vallet, D. Mele, M. Rosticher, T. Taniguchi, K. Watanabe, E. Bocquillon, G. Feve, J. M. Berroir, C. Voisin, J. Cayssol, M. O. Goerbig, J. Troost, E. Baudin, B. Placais
Summary: Researchers have achieved a mesoscopic variant of the Schwinger effect in graphene transistors, which involves the creation of matter by electric fields. By conducting transport measurements, they observed universal one-dimensional Schwinger conductance at the pinch-off of the transistors. These findings enhance our understanding of current saturation limits in ballistic graphene and open up new directions for quantum electrodynamic experiments in the laboratory.
Article
Physics, Multidisciplinary
Jiang-Xiazi Lin, Phum Siriviboon, Harley D. Scammell, Song Liu, Daniel Rhodes, K. Watanabe, T. Taniguchi, James Hone, Mathias S. Scheurer, J. I. A. Li
Summary: A superconducting diode effect is observed in twisted trilayer graphene at zero magnetic field, indicating the coexistence of superconductivity and time-reversal symmetry breaking. This non-reciprocal behavior can be controlled by adjusting carrier density, twist angle, or applying a magnetic field.
Article
Materials Science, Multidisciplinary
Wenjing Miao, Xinwen Gai, Jing Yu, Ying Jin, Jingang Wang
Summary: This study investigated the optical absorption and electronic properties of graphene nanosheets encapsulated in h-BN at different twisted angles. The results showed a red shift in absorption peak and a decrease in molar absorption coefficient for the encapsulated graphene nanosheets compared to monolayer graphene. Furthermore, the twisted angles affected the distribution breadth of electron hole pair density and charge density difference.
MATERIALS RESEARCH EXPRESS
(2022)
Article
Chemistry, Multidisciplinary
Zhe Kong, Pengzhen Zhang, Jiangxing Chen, Hanxing Zhou, Xuanchao Ma, Hongbo Wang, Jia-Wei Shen, Li-Jun Liang
Summary: The study demonstrates that GQDs of different shapes can translocate through lipid membranes within nanoseconds and tend to stabilize in the middle of the cell membrane. Additionally, GQDs do not induce notable damage to the cell membrane, indicating their potential as biomedical materials.
Article
Physics, Multidisciplinary
Priya Tiwari, Saurabh Kumar Srivastav, Aveek Bid
Summary: This study reports the discovery of electric-field-induced transition from a topologically trivial to a topologically nontrivial band structure in an atomically sharp heterostructure of bilayer graphene (BLG) and single-layer WSe2, based on the theoretical predictions of Gmitra and Fabian. The analysis shows that this bandstructure evolution arises from an interplay between proximity-induced strong spin-orbit interaction (SOI) and the layer polarizability in BLG. The results demonstrate the potential for achieving highly tunable devices based on the valley Zeeman effect in dual-gated two-dimensional materials.
PHYSICAL REVIEW LETTERS
(2021)
Article
Nanoscience & Nanotechnology
Qingrui Dong, Xiaoyu Yin, Chunxiang Liu
Summary: This study analyzes the energy difference of graphene quantum dots to investigate the control of spin switches using weak and strong electric fields, finding that graphene quantum dots of larger size can serve as qubits under a weak electric field.
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
(2021)
Article
Materials Science, Multidisciplinary
Yadong Wei, Weiqi Li, Yongyuan Jiang, Jinluo Cheng
Summary: Theoretical investigation on one-color injection currents and shift currents in zigzag graphene nanoribbons reveals that these two currents can be separately excited by specific light polarization. Numerical calculations based on a tight binding model show peaks associated with optical transitions between different subbands, which can be effectively controlled by the static electric field. The results provide a physical basis for realizing passive optoelectronic devices based on graphene nanoribbons.
Article
Materials Science, Multidisciplinary
Jing Li, Yang Cui, Lin Zhang
Summary: In this study, self-consistent charge density functional tight-binding simulations were conducted to investigate the effects of applied electrical fields on the adsorption behaviors of C60 on perfect or defective graphene. The results showed that the applied electrical field can adjust the physical adsorption of C60 on graphene, and also modulate the adsorption behaviors on graphene with a vacancy.
DIAMOND AND RELATED MATERIALS
(2022)
Article
Materials Science, Multidisciplinary
P. Elliott, N. Singh, K. Krieger, E. K. U. Gross, S. Sharma, J. K. Dewhurst
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
(2020)
Article
Physics, Multidisciplinary
T. Mueller, S. Sharma, E. K. U. Gross, J. K. Dewhurst
PHYSICAL REVIEW LETTERS
(2020)
Article
Chemistry, Multidisciplinary
Philippe Scheid, Sangeeta Sharma, Gregory Malinowski, Stephane Mangin, Sebastien Lebegue
Summary: This research utilized ab initio real-time time-dependent density functional theory to study the impact of optical and extreme ultraviolet circularly polarized femtosecond pulses on the magnetization dynamics of ferromagnetic materials. It was found that the light-induced helicity-dependent reduction of magnetization was more pronounced in the XUV regime, where 3p semicore states were involved. The study also separated the effects of absorption and the inverse Faraday effect on magnetization dynamics, showing that the former had a greater impact overall, especially in the XUV regime.
Article
Physics, Multidisciplinary
E. Golias, I Kumberg, I Gelen, S. Thakur, J. Goerdes, R. Hosseinifar, Q. Guillet, S. Sharma, C. Schuessler-Langeheine, N. Pontius, W. Kuch, K. Dewhurst
Summary: The study provides evidence for an ultrafast optically induced ferromagnetic alignment of antiferromagnetic Mn in Co/Mn multilayers. The transient ferromagnetic signal is observed at the arrival of the pump pulse at the Mn L-3 resonance, indicating a timescale comparable to the excitation duration. Theoretical calculations suggest that the emergence of this transient ferromagnetic state is due to the imbalanced population of Mn unoccupied states caused by the Co interface.
PHYSICAL REVIEW LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Abhijeet Kumar, Denis Yagodkin, Nele Stetzuhn, Sviatoslav Kovalchuk, Alexey Melnikov, Peter Elliott, Sangeeta Sharma, Cornelius Gahl, Kirill Bolotin
Summary: The study utilized a TMD heterostructure MoS2-MoSe2 to investigate spin/valley polarization and relaxation mechanisms of photoexcited carriers, revealing that the carriers maintain their spin across the interface and exhibit significantly different depolarization rates for electrons and holes. The findings offer insights into the spin/valley dynamics of photoexcited carriers and establish TMD heterostructures as generators of spin currents in spin/valleytronic devices.
Article
Optics
S. Sharma, P. Elliott, S. Shallcross
Summary: This study reveals that valley coupling is a general effect on femtosecond time scales, not limited to circularly polarized light. Two time-separated linearly polarized pulses can provide almost complete control over valley excitation, with the pulse time difference and polarization vectors being key parameters.
Article
Multidisciplinary Sciences
Sangeeta Sharma, Sam Shallcross, Peter Elliott, J. Kay Dewhurst
Summary: In the field of femtomagnetism, researchers have discovered the phenomenon of femto-phono-magnetism, where phonon excitations control magnetic order at ultrafast times. Through theoretical simulations, they have identified dominant nonadiabatic spin-phonon coupled modes that affect early time spin dynamics. Activating these phonon modes in iron-platinum leads to increased loss of moment.
Article
Multidisciplinary Sciences
Sangeeta Sharma, Peter Elliott, Samuel Shallcross
Summary: This study demonstrates that a hencomb pulse, which combines circularly polarized optical frequency pulse and linearly polarized THz pulse, can generate precisely tailored spin currents and valley currents in 2D materials. The control over these currents can be achieved by tuning the frequency and polarization vector of the light components. This result opens up a pathway for light control over spin/valley current states at ultrafast times.
Article
Materials Science, Multidisciplinary
C. -Yu Wang, S. Sharma, E. K. U. Gross, J. K. Dewhurst
Summary: This article extends the definition of Born effective charge to the dynamical regime by calculating the Fourier transform of the total electronic current divided by the Fourier transform of the velocity of a particular nucleus. The calculated dynamical Born effective charges exhibit a rich response function and prominent resonance peaks, while also being able to reproduce the usual static Born effective charges.
Article
Materials Science, Multidisciplinary
S. Shallcross, C. V. Korff Schmising, P. Elliott, S. Eisebitt, J. K. Dewhurst, S. Sharma
Summary: This study investigates the microscopic processes of ultrafast demagnetization using first-principles dynamical simulations. The experimentally observed energy peak shift can be explained by laser-induced changes in band occupation, and different behaviors are observed for cobalt and nickel.
Article
Materials Science, Multidisciplinary
C. -Yu Wang, S. Sharma, T. Muller, E. K. U. Gross, J. K. Dewhurst
Summary: With the application of Wick's theorem, this study derives a set of equations to incorporate small amplitude quantum nuclear dynamics in solid-state calculations. The derived equations involve noninteracting fermionic and bosonic Hamiltonians, which are solved self-consistently and require Bogoliubov transformations for diagonalization. The method has been implemented in an all-electron code and successfully predicts various properties of materials.
Article
Materials Science, Multidisciplinary
S. Theil, M. Fleischmann, R. Gupta, F. Rost, F. Wullschlaeger, S. Sharma, B. Meyer, S. Shallcross
Summary: The study establishes a general relation between the stacking vector and Chern index in bilayer graphene, demonstrating the robustness of the topological physics to lattice relaxations. The research also highlights the identical Chern index maps of ideal and relaxed minimally twisted bilayer graphene, despite their distinct appearances.
Article
Materials Science, Multidisciplinary
J. K. Dewhurst, S. Shallcross, P. Elliott, S. Eisebitt, C. V. Korff Schmising, S. Sharma
Summary: Researchers have demonstrated the transfer of spin angular momentum to orbital angular momentum during ultrafast demagnetization, and proposed using thin film cobalt structure in experiments to observe the fast momentum transfer process clearly.
Article
Materials Science, Multidisciplinary
N. Singh, P. Elliott, J. K. Dewhurst, S. Sharma
Summary: This study demonstrates how fundamental properties of magnons can be manipulated using femtosecond laser pulses, such as element-selective destruction, delay-dependent freezing, and frequency renormalization. Harnessing these processes could significantly accelerate the development of magnonic devices.
Article
Materials Science, Multidisciplinary
Q. Z. Li, P. Elliott, J. K. Dewhurst, S. Sharma, S. Shallcross
Summary: This paper demonstrates an excellent method for describing momentum-resolved charge excitation in monolayer graphene using transient electron momentum density, with results showing excellent agreement with conduction band occupancy obtained from advanced theoretical calculations. It confirms that simple model-based tight-binding approaches can provide an excellent description for laser-induced electron dynamics in graphene, even under intense laser pulses.