Article
Chemistry, Physical
Vanessa Meschke, Prashun Gorai, Vladan Stevanovic, Eric S. Toberer
Summary: By searching and classifying materials from two different crystal structure databases, approximately 500 compounds with a transition metal or rare-earth Kagome sublattice were identified. An extensive analysis of the chemical and structural trends revealed three types of Kagome sheet stacking and multiple classes of magnetic complexity. Rapid screening of magnetic properties using density functional theory rediscovered some materials previously studied for low-temperature magnetic behavior, as well as identified three materials that appear to be unexplored for their magnetic properties.
CHEMISTRY OF MATERIALS
(2021)
Article
Materials Science, Multidisciplinary
Johannes Richter, Oleg Derzhko, Juergen Schnack
Summary: Over the last decade, the interest in the spin-1/2 Heisenberg antiferromagnet (HAF) on the square kagome lattice has been growing. This model system is a prominent example of quantum magnetism with a quantum paramagnetic ground state, flat-band physics near the saturation field, and quantum scars. Recent numerical investigations have revealed a gapless spin liquid in the square kagome magnet. The study also provides insights into specific heat, entropy, and susceptibility, revealing low-temperature shoulder below the major maximum and a change in curvature just at a specific temperature, attributed to low-lying singlet excitations and the singlet-triplet gap.
Article
Chemistry, Multidisciplinary
Wan-Hsin Chen, Chin-Hsuan Chen, Guan-Hao Chen, Wei-Chuan Chen, Fu-Xiang Rikudo Chen, Pei-Jung Chen, Chun-Kai Ku, Chang-Tsan Lee, Naoya Kawakami, Jia-Ying Li, Iwao Matsuda, Wen-Hao Chang, Juhn-Jong Lin, Chien-Te Wu, Chung-Yu Mou, Horng-Tay Jeng, Shu-Jung Tang, Chun-Liang Lin
Summary: In this work, a buckled plumbene-Au Kagome superstructure grown by depositing Au on Pb(111) is investigated, which not only has an enhanced superconducting critical temperature (T-c) with respect to that of a monolayer Pb but also possesses a higher value than what owned by a bulk Pb substrate. By combining angle-resolved photoemission spectroscopy with density functional theory, the monolayer Au-intercalated low-buckled plumbene sandwiched between the top Au Kagome layer and the bottom Pb(111) substrate is confirmed and the electron-phonon coupling-enhanced superconductivity is revealed. This work demonstrates that a buckled plumbene-Au Kagome superstructure can enhance superconducting T-c and Rashba effect, effectively triggering the novel properties of a plumbene.
Article
Materials Science, Multidisciplinary
Quinn D. Gibson, Ramzy Daou, Marco Zanella, Jonathan Alaria, Matthew J. Rosseinsky
Summary: The magnetic, electronic, and thermal properties of Fe3Ge2Sb single crystals, a derivative of the hexagonal FeGe structure, are investigated. Fe3Ge2Sb exhibits similar properties to FeGe, except for the lack of a charge density wave transition. This makes Fe3Ge3-xSbx compounds a good choice for studying various physical effects in kagome metals.
Article
Materials Science, Multidisciplinary
Johannes Richter, Jurgen Schnack
Summary: The spin-1/2 Heisenberg antiferromagnet on the square-kagome (SK) lattice has been a subject of interest in quantum magnetism due to its high frustration. Recent discoveries of SK spin-liquid compounds further motivate theoretical studies of this model. This study investigates the temperature dependence of various thermodynamic properties of the SK antiferromagnet with different strength of nearest-neighbor bonds J1 and J2. The findings reveal different ground states and low-temperature behaviors depending on the ratio of J2/J1.
Article
Materials Science, Multidisciplinary
Yasir Iqbal, Francesco Ferrari, Aishwarya Chauhan, Alberto Parola, Didier Poilblanc, Federico Becca
Summary: In this study, the ground-state phase diagram of the J(1) - J(2) Heisenberg model on a Kagome lattice was assessed using Gutzwiller-projected fermionic wave functions. The accuracy of the U(1) Dirac state, describing the exact ground state, improves with the presence of a small antiferromagnetic superexchange J(2), leading to stability of a gapless spin liquid. For small ferromagnetic values of J(2)/J(1), the U(1) Dirac state remains stable against various perturbations but deteriorates on small systems, eventually giving way to a magnetically ordered state with root 3 x root 3 periodicity. Additionally, evidence of a first-order transition in the ferromagnetic J(2) regime is shown at J(2)/J(1) = -0.065(5).
Article
Materials Science, Multidisciplinary
Tristan Lugan, Ludovic D. C. Jaubert, Masafumi Udagawa, Arnaud Ralko
Summary: In this study, we employ Schwinger boson mean-field theory to investigate the quantum spin-1/2 model of the kagome antiferromagnet with first, second, and third neighbor exchanges (J1, J2, J3). By using two different rewritings of the Hamiltonian, we gain insight into the origin of the phase transitions. The system exhibits different phases, including spin liquid and long-range chiral order, in certain parameter ranges.
Article
Materials Science, Multidisciplinary
J. S. R. McCoombs, A. Zelenskiy, M. L. Plumer, B. W. Southern, T. L. Monchesky
Summary: We conducted a symmetry analysis of the ABC-stacked kagome planes of Mn atoms in the L12 Mn3X and antiperovskite Mn3AB alloys. Apart from the known single-ion-anisotropy and Kitaev-type anisotropic exchange, we discovered a staggered Dzyaloshinskii-Moriya interaction and gamma-type anisotropic exchange between nearest-neighbor spins. These new terms do not affect the ground state energy of the 120 degrees spin structures but become apparent in spin-wave excitations. We demonstrated the effects through calculations of inelastic neutron-scattering cross sections, suggesting experimental methods to investigate the existence and strengths of these cloaked interactions.
Article
Materials Science, Multidisciplinary
Yongchang Li, Chang Liu, Guo-Dong Zhao, Tao Hu, Wei Ren
Summary: In this study, we theoretically predict the manipulation of ferroelectric and ferromagnetic properties in 2D materials using Ti3X8 compounds. By altering lattice structures and applying electric fields, the coupling of magnetism and ferroelectricity is achieved in bilayer Ti3X8, leading to magnetic configuration transformations. This research expands the possibilities for realizing 2D multiferroics and magnetoelectric effects.
Article
Materials Science, Multidisciplinary
A. Ochiai, N. Kabeya, K. Maniwa, M. Saito, S. Nakamura, K. Katoh
Summary: The magnetic properties of CeZn3P3 were studied, revealing a slightly deformed crystal structure even at room temperature. CeZn3P3 maintains its deformed structure from high temperatures to extremely low temperatures, showing magnetic order below T-N = 0.8K. The magnetic phase diagram below T-N resembles a magnetic flower blooming on the c plane, possibly related to a quasi S = 1/2 spin system and an orbital component.
Article
Materials Science, Multidisciplinary
Z. X. Wang, Q. Wu, Q. W. Yin, C. S. Gong, Z. J. Tu, T. Lin, Q. M. Liu, L. Y. Shi, S. J. Zhang, D. Wu, H. C. Lei, T. Dong, N. L. Wang
Summary: Recent research on the kagome lattice metal AV(3)Sb(5) (A = K, Rb, Cs) family indicates the coexistence of superconductivity, charge density wave (CDW), and peculiar properties arising from a topological nontrivial electronic structure. The results suggest that the CDW order in this family is very different from a conventional CDW condensate, with the excited quasiparticle relaxation dynamics explained by the formation of a temperature-dependent energy gap below the phase transition.
Article
Materials Science, Multidisciplinary
Hong Li, Tao Li
Summary: The extreme frustration in the kagome antiferromagnet allows for the realization of numerous closely competing magnetic phases. Through simulation and calculation, it has been found that in a certain region, there is a competition between q = 3 and q = 4 Potts order, which cannot be explained by the conventional order-by-disorder mechanism. This region may host a nematic spin liquid ground state with an anisotropic ring structure.
Article
Chemistry, Multidisciplinary
Sen Shao, Jia-Xin Yin, Ilya Belopolski, Jing-Yang You, Tao Hou, Hongyu Chen, Yuxiao Jiang, Md Shafayat Hossain, Mohammad Yahyavi, Chia-Hsiu Hsu, Yuan Ping Feng, Arun Bansil, M. Zahid Hasan, Guoqing Chang
Summary: Recent experiments report the existence of a charge density wave (CDW) in the antiferromagnet FeGe, but the nature of the charge ordering and associated structural distortion is still unclear. By examining the structural and electronic properties of FeGe, our study reveals that the 2 x 2 x 1 CDW is likely due to Fermi surface nesting of hexagonal-prism-shaped kagome states. We find that the distortion in FeGe mainly occurs in the positions of Ge atoms in the kagome layers rather than Fe atoms. Through calculations and modeling, we demonstrate that this unconventional distortion is driven by the intertwining of magnetic exchange coupling and CDW interactions in this kagome material. The movement of Ge atoms also enhances the magnetic moment of the Fe kagome layers.
Article
Multidisciplinary Sciences
S. Spachmann, P. Berdonosov, M. Markina, A. Vasiliev, R. Klingeler
Summary: High-resolution capacitance dilatometry was conducted on single crystals of Cu3Bi(SeO3)(2)O2Cl, revealing pronounced magnetoelastic coupling at 26.4(3) K and moderate effects of uniaxial pressure on T-N along the a, b, and c axes. Competing interactions were observed below 22 K. The structural phase transition at Ts showed higher sensitivity to uniaxial pressure than T-N, and magnetostriction and magnetization measurements indicated a linear magnetoelastic coupling and mixed phase behavior.
SCIENTIFIC REPORTS
(2022)
Article
Materials Science, Multidisciplinary
Mutsuki Saito, Ryunosuke Takagishi, Nobuyuki Kurita, Masari Watanabe, Hidekazu Tanaka, Ryuji Nomura, Yoshiyuki Fukumoto, Kazuhiko Ikeuchi, Ryoichi Kajimoto
Summary: Cs2Cu3SnF12 and Rb2Cu3SnF12 are two spin-1/2 antiferromagnets with different structures, and their magnetic excitation structures were investigated using inelastic neutron scattering. Four single-magnon excitation modes were observed in Cs2Cu3SnF12, and a broad excitation continuum was found. In Rb2Cu3SnF12, singlet-triplet excitations from the pinwheel VBS state were confirmed, along with ghost modes caused by the enlargement of the chemical unit cell.
Article
Physics, Multidisciplinary
Pyeongjae Park, Kisoo Park, Taehun Kim, Yusuke Kousaka, Ki Hoon Lee, T. G. Perring, Jaehong Jeong, Uwe Stuhr, Jun Akimitsu, Michel Kenzelmann, Je-Geun Park
PHYSICAL REVIEW LETTERS
(2020)
Article
Multidisciplinary Sciences
Allen Scheie, Jonas Kindervater, Shu Zhang, Hitesh J. Changlani, Gabriele Sala, Georg Ehlers, Andre Heinemann, Gregory S. Tucker, Seyed M. Koohpayeh, Collin Broholm
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2020)
Article
Multidisciplinary Sciences
Wesley T. Fuhrman, Andrey Sidorenko, Jonathan Haenel, Hannes Winkler, Andrey Prokofiev, Jose A. Rodriguez-Rivera, Yiming Qiu, Peter Blaha, Qimiao Si, Collin L. Broholm, Silke Paschen
Summary: The study investigates the Kondo semimetal CeRu4Sn6 by magnetic susceptibility, specific heat, and inelastic neutron scattering experiments, revealing that this compound is quantum critical without tuning and that temperature is the only energy scale in the criticality.
Article
Chemistry, Physical
Jonathan Gaudet, Hung-Yu Yang, Santu Baidya, Baozhu Lu, Guangyong Xu, Yang Zhao, Jose A. Rodriguez-Rivera, Christina M. Hoffmann, David E. Graf, Darius H. Torchinsky, Predrag Nikolic, David Vanderbilt, Fazel Tafti, Collin L. Broholm
Summary: In NdAlSi, Weyl fermions mediate a helical incommensurate spin density wave, serving as a rare example of Weyl-mediated collective phenomena. This material demonstrates unique electronic properties of Weyl semimetals and reveals collective magnetism associated with Weyl fermions through techniques such as neutron diffraction.
Article
Multidisciplinary Sciences
Yishu Wang, T. Reeder, Y. Karaki, J. Kindervater, T. Halloran, N. Maliszewskyj, Yiming Qiu, J. A. Rodriguez, S. Gladchenko, S. M. Koohpayeh, S. Nakatsuji, C. Broholm
Summary: The text discusses the formation of low-energy states by ferromagnetically interacting Ising spins on a specific lattice structure, and investigates the process of spin flip leading to fractionalization of magnetic monopoles. Through experiments, the microscopic mechanisms of magnetic relaxation in spin ice at different temperatures were revealed.
Article
Chemistry, Physical
Xinshu Zhang, Yuanyuan Xu, T. Halloran, Ruidan Zhong, C. Broholm, R. J. Cava, N. Drichko, N. P. Armitage
Summary: By using time-domain terahertz spectroscopy, we observed the characteristics of a quantum spin liquid in the cobalt-based magnet BaCo2(AsO4)(2) over a wide range of temperatures and fields. The application of a magnetic field can suppress magnetic ordering and induce a spin-polarized state. A possible field-induced quantum spin liquid was observed under a specific out-of-plane magnetic field.
Article
Materials Science, Multidisciplinary
Huiyuan Man, Alireza Ghasemi, Moein Adnani, Maxime A. Siegler, Elaf A. Anber, Yufan Li, Chia-Ling Chien, Mitra L. Taheri, Ching-Wu Chu, Collin L. Broholm, Seyed M. Koohpayeh
Summary: Little is known about the magnetism of A(2)B(2)O(7) monoclinic layered perovskites. The study investigates the chemical phase stability, structure, and magnetic properties of Pr2Ti2O7. It is found that Pr2Ti2O7 forms a singlet ground state quantum paramagnet that does not undergo any magnetic phase transitions.
PHYSICAL REVIEW MATERIALS
(2023)
Article
Materials Science, Multidisciplinary
X. Y. Li, D. Reig-i-Plessis, P-F Liu, S. Wu, B-T Wang, A. M. Hallas, M. B. Stone, C. Broholm, M. C. Aronson
Summary: Sc3Mn3Al7Si5 is a rare example of a correlated metal with a kagome lattice formed by Mn moments. The absence of magnetic ordering at low temperatures suggests strong magnetic fluctuations due to geometrical frustration. Inelastic neutron scattering measurements showed that phonon scattering dominates at energies from 20-50 meV, with a weak magnetic signal detected at energies less than 10 meV only at the lowest temperatures.
Article
Materials Science, Multidisciplinary
A. Scheie, M. Sanders, Xin Gui, Yiming Qiu, T. R. Prisk, R. J. Cava, C. Broholm
Summary: The study presents the low-temperature magnetic properties of Nd2ScNbO7, including susceptibility, magnetization, elastic and inelastic neutron scattering. The findings indicate a unique fluctuating magnetic ground state that resembles a spin liquid but may have other underlying mechanisms. The presence of static electronic moments and suppression of nuclear Schottky anomaly suggest complex magnetic interactions influenced by disorder.
Article
Materials Science, Multidisciplinary
Hung-Yu Yang, Bahadur Singh, Jonathan Gaudet, Baozhu Lu, Cheng-Yi Huang, Wei-Chi Chiu, Shin-Ming Huang, Baokai Wang, Faranak Bahrami, Bochao Xu, Jacob Franklin, Ilya Sochnikov, David E. Graf, Guangyong Xu, Yang Zhao, Christina M. Hoffman, Hsin Lin, Darius H. Torchinsky, Collin L. Broholm, Arun Bansil, Fazel Tafti
Summary: Research on novel electromagnetic responses such as the anomalous Hall effect in ferromagnetic Weyl semimetals shows promise. CeAlSi, a FM-WSM material, stands out for its noncentrosymmetric lattice, noncollinear FM ordering, and novel AHE that is anisotropic between the easy and hard magnetic axes. This material also exhibits large FM domains, offering potential for exploring device applications and the interplay between Weyl nodes and FM domain walls.
Article
Physics, Multidisciplinary
Michael E. Valentine, Tomoya Higo, Yusuke Nambu, Dipanjan Chaudhuri, Jiajia Wen, Collin Broholm, Satoru Nakatsuji, Natalia Drichko
PHYSICAL REVIEW LETTERS
(2020)
Article
Materials Science, Multidisciplinary
Christian Wessler, Bertrand Roessli, Karl W. Kraemer, Bernard Delley, Oliver Waldmann, Lukas Keller, Denis Cheptiakov, Hans B. Braun, Michel Kenzelmann
NPJ QUANTUM MATERIALS
(2020)
Article
Materials Science, Multidisciplinary
J. Lohr, A. L. Larralde, J. Curiale, R. Sanchez, J. Campo, G. J. Cuello, D. Sheptyakov, L. Keller, M. Kenzelmann, G. Aurelio
Article
Materials Science, Multidisciplinary
Y. Gritsenko, S. Mombetsu, P. T. Cong, T. Stoeter, E. L. Green, C. Salazar Mejia, J. Wosnitza, M. Ruminy, T. Fennell, A. A. Zvyagin, S. Zherlitsyn, M. Kenzelmann
Article
Materials Science, Multidisciplinary
S. Shin, V Pomjakushin, L. Keller, P. F. S. Rosa, U. Stuhr, C. Niedermayer, R. Sibille, S. Toth, J. Kim, H. Jang, S-K Son, H-O Lee, T. Shang, M. Medarde, E. D. Bauer, M. Kenzelmann, T. Park