期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 5, 期 19, 页码 3325-3329出版社
AMER CHEMICAL SOC
DOI: 10.1021/jz501609e
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资金
- European Commission ERC [278912]
- Robert A. Welch Foundation [F-1464]
- National Science Foundation [CHE-1308813]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1308813] Funding Source: National Science Foundation
Pyrene chromophores were attached to silicon nanocrystals (SiNCs) with diameters of 2.6 and 5.0 nm to provide light-harvesting antennae for enhanced optical absorption. Efficient energy transfer from the pyrene moieties to the SiNCs was observed to induce bright visible (2.6 nm) or near-infrared (NIR) (5.0 nm) photoluminescence (PL). The 5.0 nm diameter pyrene-derivatized SiNCs exhibited NIR PL emission that was insensitive to dioxygen, with a 40% quantum yield and long lifetime (hundreds of mu s).
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