期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 1, 期 16, 页码 2455-2458出版社
AMER CHEMICAL SOC
DOI: 10.1021/jz1008888
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资金
- Robert A Welch Foundation [A-1405]
- Office of Science, Office of Basic Energy Science. Division of Chemical Science, Geoscience and Bioscience [FG0204 ER15593]
We report correlated state distributions arising from NO3 photolysis at 588 nm using velocity map ion imaging.-State-selected NO images reveal clear evidence for two dissociation pathways for the NO 02 channel Vibrationally excited 02 (31.-g, v = 5-10) is formed in coincidence with low rotational states of NO (2n) in the dominant mechanism We also observe a small channel consisting of low vibrational levels of 02 (34, v = 0-4) coincident with high NO rotational states We discuss the results in the context of the recent studies of formaldehyde dissociation and postulate the involvement of roaming-type dynamics. SECTION Dynamics, Clusters, Excited States
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