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Spatially Resolved Thermodynamics of the Partially Ionized Exciton Gas in GaAs

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PHYSICAL REVIEW LETTERS
卷 114, 期 22, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.114.227402

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  1. DFG [SPP1285 OS98/9-3]

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We report on the observation of macroscopic free exciton photoluminescence (PL) rings that appear in spatially resolved PL images obtained on a high purity GaAs sample. We demonstrate that a spatial temperature gradient in the photocarrier system, which is due to nonresonant optical excitation, locally modifies the population balance between free excitons and the uncorrelated electron-hole plasma described by the Saha equation and accounts for the experimentally observed nontrivial PL profiles. The exciton ring formation is a particularly instructive manifestation of the spatially dependent thermodynamics of a partially ionized exciton gas in a bulk semiconductor.

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