期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 79, 期 11, 页码 5282-5286出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo5008652
关键词
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资金
- National Natural Science Foundation of China [NSF 21002078, 21372184]
- State Education Ministry Scientific Research Foundation for Returned Overseas Chinese Scholars
- Shaanxi Province Technology Foundation for Selected Overseas Chinese
A strategy to the 6-5-6 tricyclic scaffold of taiwaniaquinoids was established on the basis of a one-pot thermal ring expansion/4 pi-electrocyclization process. The efficiency of this methodology has been demonstrated through its application in the total synthesis of taiwaniaquinone H, which has been accomplished in three steps and 14% overall yield in a protecting-group-free manner starting from commercially available materials.
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