期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 79, 期 18, 页码 8768-8773出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo501601u
关键词
-
资金
- National Natural Science Foundation of China [21372068, J1210040, J1103312]
The development of a novel intermolecular oxidative C-H alkoxylation of aniline derivatives is described under metal-free conditions with high reaction rates at ambient temperature. In the presence of an I(III) oxidant, a range of aldehydes, anilines, and alcohol substrates undergo three-component coupling to produce synthetically useful alkoxyl-substituted N-arylimines. The preliminary mechanism investigations revealed that the transformation proceeds via imines as intermediates.
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