期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 78, 期 16, 页码 7777-7784出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo401091w
关键词
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资金
- NSF [CHE-1152491, CHE-1213578]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1152491, 1213578] Funding Source: National Science Foundation
Spatial orthogonality of the two independently addressable pi-systems in alkynes can be used for the design and control of metal-free cascade transformations. Examples include ionic chemistry of neutral hydrocarbons, preparation of radicals without radical initiators, generation of excited states without light, 1,2-dicarbene reactivity of alkynes in boomerang radical processes, selective conversion of alkynes into carbonyl compounds, and full disassembly of the alkyne moiety.
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