期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 76, 期 17, 页码 7186-7194出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo201214x
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资金
- NSF
- ACS-PRF
- NCSA
- University of California, Davis
- National Science Foundation [CHE-0847358]
- 3M Corporation
- Bradford Borge Chemistry Fellowship
- Department of Education
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0953464] Funding Source: National Science Foundation
The fundamental properties of a series of organic monosilanols, silanediols, disiloxanediols, and known hydrogen-bonding organocatalysts have been examined in the gas phase using computational and experimental mass spectrometry methods. The organosilicon diol molecules contain dual hydrogen-bonding groups that were designed as potential hosts and hydrogen-bonding catalysts. Newly measured acidities are reported, and implications regarding solvent effects, catalysis, and molecular recognition are discussed.
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