期刊
PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES
卷 14, 期 12, 页码 2147-2150出版社
SPRINGERNATURE
DOI: 10.1039/c5pp00259a
关键词
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Proton-coupled electron transfer (PCET) plays a central role in photosynthesis and potentially in solar-to-fuel systems. We report a spectroscopy study on a phenol-pyrrolidino[60]fullerene. Quenching of the singlet excited state from 1 ns to 250 ps is assigned to PCET. A H/D exchange study reveals a kinetic isotope effect (KIE) of 3.0, consistent with a concerted PCET mechanism.
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