期刊
JOURNAL OF NANOPARTICLE RESEARCH
卷 16, 期 10, 页码 -出版社
SPRINGER
DOI: 10.1007/s11051-014-2635-4
关键词
Carbon quantum dots; Photocatalysts; Nanocomposites; Silica
资金
- National Natural Science Foundation of China [21201070, 51202079, 21401062]
- Natural Science Fund of Jiangsu Province [BK2012665, BK20141247, BK20140447]
- High School Science Research Key Project of Jiangsu Province [11KJA4 30008]
- University Science Research Project of Jiangsu Province [13KJB430005]
- Jiangsu Overseas Research & Training Program for University Prominent Yong & Middle-aged Teachers and Presidents
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- Public Science and Technology Research Funds Projects of Ocean [201305007]
It is also well known that naked SiO2 is not an efficient photocatalyst due to its relatively large band gap, which could only absorb short-wave ultraviolet light. In this report, SiO2/carbon quantum dot (SiO2/CQD, about 4 nm) nanocomposites were successfully prepared by one-step thermal method using tetraethylorthosilicate (TEOS) as the source of both silicon and carbon. The nanocomposites were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), and X-ray photoelectron spectroscopy (XPS). These nanocomposites exhibit higher photocatalytic activity for rhodamine B (RhB) degradation than C-doped SiO2 and pure SiO2 nanoparticles under near-UV light irradiation at room temperature in air. In the present catalyst system, CQD play two important roles for the enhanced photocatalytic activity of SiO2/CQD nanocomposites. It is expected that these novel, environmentally friendly and highly photoactive SiO2/CQD nanocomposites may promote practical applications of photocatalysts and provide an effective approach to high-efficiency complex catalyst design.
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