期刊
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL
卷 289, 期 1-2, 页码 44-48出版社
ELSEVIER
DOI: 10.1016/j.molcata.2008.04.011
关键词
CH bond activation; homogeneous catalyst; heterogeneous catalyst; dehydrogenation; palladium complexes
A series of new palladium(II) complexes with heteroatomic chelating ligands (carboxylates and alcoholates) was synthesized. The catalytic activities of the palladium complexes were successfully tested for catalytic CH-activation reactions of cyclooctane. They gave TONs of 2.6-26.5 (300 degrees C, 16 h) in homogeneous solution and 4.6-21.4 (400 degrees C, 5 h) in heterogeneous reactions. (C) 2008 Elsevier B.V. All rights reserved.
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