期刊
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
卷 29, 期 3, 页码 221-224出版社
JOURNAL MATER SCI TECHNOL
DOI: 10.1016/j.jmst.2013.01.006
关键词
Photoluminescence; Silicon nanocrystals; Epoxy; Silicone; Quantum yield; External quantum efficiency
资金
- National Natural Science Foundation of China [50902122, 50832006]
- R&D Program of Ministry of Education of China [62501040202]
- Innovation Team Project of Zhejiang Province, China [2009R50005]
- Basic Funding for Research at Zhejiang University, China [2011FZA4005]
- Major Scientific program of Zhejiang Province, China [2009C01024-2]
Naturally oxidized freestanding silicon nanocrystals (Si NCs) are incorporated in commonly used encapsulating materials to explore the photoluminescent application of Si NCs in device structures such as solid-state lighting light-emitting diodes (LEDs) and solar cells. The quantum yield of Si NCs before the incorporation has reached about 45% at the excitation wavelength of 370 nm without any special surface modification. It is found that medium loadings, e.g., 5 wt% of Si NCs in encapsulating materials help to obtain high external quantum efficiency (EQE) of the mixtures of Si NCs and encapsulating materials. The curing of encapsulating materials significantly reduces EQE. Among all the encapsulating materials investigated in this work, silicone-OE6551 enables the highest EQE (21% at excitation wavelength lambda(ex) = 370 nm) after curing. Based on current findings, we have discussed the continuous efforts to advance the photoluminescent application of Si NCs.
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