期刊
JOURNAL OF MATERIALS CHEMISTRY
卷 22, 期 3, 页码 816-819出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1jm14555j
关键词
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资金
- National Research Foundation of Korea (NRF) [2E22111]
- Ministry of Education, Science, and Technology [2011K000592]
We report on the successful conjugation of C-60 molecules on the surface of ZnO quantum dots (QDs) and their application in multilayer structured ultraviolet (UV) photovoltaic (PV) devices. In situ growth of C-60 on the surface of ZnO QDs with a core-shell structure was realized via a mild solution-process method, which resulted in an improvement in photo-induced charge separation and transport of carriers to the collecting electrodes in a fabricated device. The conjugation of the C-60 with ZnO QDs leads to a PL quenching of about 99.8%, which can be attributed to an efficient transfer of photo-induced electrons from the ZnO QDs to the C-60 through a Zn-O-C chemical bonding. UV PV cells with ZnO-C-60 core-shell QDs as an active layer and fabricated through an all layer simple chemical method exhibit high power conversion efficiency as much as about 3.02%.
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