期刊
JOURNAL OF LUMINESCENCE
卷 132, 期 3, 页码 743-749出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jlumin.2011.11.011
关键词
Up conversion; Nano particles; Energy transfer effects; Imaging
类别
资金
- Div Of Chem, Bioeng, Env, & Transp Sys
- Directorate For Engineering [0930170] Funding Source: National Science Foundation
The effects of Yb3+ doping on up conversion in Yb3+-Er3+ co-doped cerium oxide nanocrystals are reported. Green emission around 545 and 560 nm attributed to the H-2(11/2), S-4(3/2)-> I-4(15/2) transitions and red emission around 660 and 680 nm due to F-4(9/2) -> I-4(15/2) transitions under 975 nm excitation were studied at room temperature. Both green and red emission intensities increase as the Yb3+ concentration increases from 0%. Emission strength starts to decrease after the Yb3+ concentration exceeds a critical amount. The green emission strength peaks around 1% Yb3+ concentration while the red emission strength peaks around 4%. An explanation of competition between different decay mechanisms is presented to account for the luminescence dependence on Vb(3+) concentration. Also, the application of up converting nanoparticles in biomedical imaging is demonstrated. (C) 2011 Elsevier B.V. All rights reserved.
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