4.7 Article

Degradation of estrone in water and wastewater by various advanced oxidation processes

期刊

JOURNAL OF HAZARDOUS MATERIALS
卷 278, 期 -, 页码 16-24

出版社

ELSEVIER
DOI: 10.1016/j.jhazmat.2014.05.078

关键词

Estrone (E1); Secondary effluent; AOP; Total organic carbon; Yeast estrogen screen assay

资金

  1. Natural Sciences and Engineering Research Council (NSERC)
  2. Trojan Technologies, Inc., Canada

向作者/读者索取更多资源

A comprehensive study was conducted to determine the relative efficacy of various advanced oxidation processes such as O-3, H2O2, UV, and combinations of UV/O-3, UV/H2O2 for the removal of estrone (E1) from pure water and secondary effluent. In addition to the parent compound (El) removal, performance of the advanced oxidation processes was characterized using removal of total organic carbon (TOC), and estrogenicity of the effluent. Although E1 removal was high for all the AOPs, intermediates formed were more difficult to degrade leading to slow TOC removal. Energy calculations and cost analysis indicated that, although UV processes have low electricity cost, ozonation is the least cost option ($ 0.34/1000 gallons) when both capital and operating costs were taken into account. Ozonation also is superior to the other tested AOPs due to higher removal of TOC and estrogenicity. The rate of E1 removal decreased linearly with the background TOC in water, however, E1 degradation in the secondary effluent from a local wastewater treatment plant was not affected significantly due to the low COD values in the effluent. (C) 2014 Elsevier B.V. All rights reserved.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.7
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Biotechnology & Applied Microbiology

Noninvasive tool for optical online monitoring of individual biomass concentrations in a defined coculture

Bertram Geinitz, Lars Rehmann, Jochen Buechs, Lars Regestein

BIOTECHNOLOGY AND BIOENGINEERING (2020)

Article Chemistry, Multidisciplinary

Cultivation Strategies of Clostridium autoethanogenum on Xylose and Carbon Monoxide Combination

Marcel Mann, Garret Munch, Lars Regestein, Lars Rehmann

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

Article Engineering, Chemical

Self-Synchronized Oscillatory Metabolism of Clostridium pasteurianum in Continuous Culture

Erin E. Johnson, Lars Rehmann

PROCESSES (2020)

Article Soil Science

Impacts of corn stover removal on carbon dioxide and nitrous oxide emissions

C. F. Drury, A. L. Woodley, W. D. Reynolds, X. M. Yang, L. A. Phillips, L. Rehmann, W. Calder

Summary: This study evaluated the impacts of removing corn stover on soil-borne CO2 and N2O emissions, finding that stover removal may decrease CO2 emissions but increase N2O emissions, with different effects observed under different tillage practices.

SOIL SCIENCE SOCIETY OF AMERICA JOURNAL (2021)

Article Agricultural Engineering

Feasibility of anaerobic digestion as a treatment for the aqueous pyrolysis condensate (APC) of birch bark

Connie Wen, Cesar M. Moreira, Lars Rehmann, Franco Berruti

BIORESOURCE TECHNOLOGY (2020)

Editorial Material Engineering, Chemical

Special Issue: Application of Advanced Oxidation Processes

Ciro Bustillo-Lecompte, Jose Colina-Marquez, Lars Rehmann

PROCESSES (2020)

Article Chemistry, Multidisciplinary

Comparison of Biobutanol Production Pathways via Acetone- Butanol-Ethanol Fermentation Using a Sustainability Exergy-Based Metric

Samir I. Meramo-Hurtado, Angel D. Gonzalez-Delgado, Lars Rehmann, Edgar Quinones-Bolanos, Mehrab Mehrvar

ACS OMEGA (2020)

Article Engineering, Chemical

Removal of phenolics from aqueous pyrolysis condensate by activated biochar

Tahereh Sarchami, Neha Batta, Lars Rehmann, Franco Berruti

Summary: This study investigated the feasibility of using pyrolytic biochar as an adsorbent for the selective removal of phenolics from aqueous pyrolysis condensate (APC). The results showed that activated soft wood (ASW) biochar had the highest efficiency and capacity for removing phenol from water solutions. The adsorption data with ASW biochar were well described by pseudo second-order equation and Freundlich model, making it a promising environmentally friendly adsorbent for phenolics removal.

CANADIAN JOURNAL OF CHEMICAL ENGINEERING (2021)

Article Chemistry, Multidisciplinary

Environmental and Exergetic Analysis of Large-Scale Production of Citric Acid-Coated Magnetite Nanoparticles via Computer-Aided Process Engineering Tools

David Alfonso Patino-Ruiz, Samir Isaac Meramo-Hurtado, Mehrab Mehrvar, Lars Rehmann, Edgar Quinones-Bolanos, Angel Dario Gonzalez-Delgado, Adriana Herrera

Summary: This study evaluates the potential environmental impacts and exergetic efficiency of scaled-up production of citric acid-coated magnetite nanoparticles. Simulations using waste reduction algorithm and Aspen Plus software show high environmental performance attributed to the generation of environmentally friendlier substances and high contributions to toxicity potentials from ethanol in waste streams. The global exergy efficiency increases with improvements in centrifuge performance, emphasizing the importance of addressing ethanol disposal in wastewater.

ACS OMEGA (2021)

Article Green & Sustainable Science & Technology

Comparative analysis of biorefinery designs based on acetone- butanol-ethanol fermentation under exergetic, techno-economic, and sensitivity analyses towards a sustainability perspective

Samir Meramo-Hurtado, Angel Gonzalez-Delgado, Lars Rehmann, Edgar Quinones-Bolanos, Mehrab Mehvar

Summary: This study presents a comprehensive assessment of two biorefinery configurations for butanol production, involving techno-economic, sensitivity, and exergetic factors. The results indicate that both configurations are economically viable alternatives, with topology 2 showing higher exergetic efficiency compared to topology 1.

JOURNAL OF CLEANER PRODUCTION (2021)

Article Agronomy

Stover harvest and tillage effects on corn seedling emergence

Ikechukwu V. Agomoh, Craig F. Drury, W. Daniel Reynolds, Alex Woodley, Xueming Yang, Lori A. Phillips, Lars Rehmann

Summary: The study showed that under continuous corn cropping system, no-tillage practice compared to conventional tillage can improve corn seedling emergence and reduce the negative impact of stover on plant growth. Stover removal from corn fields can help mitigate the effects on seedling emergence early in the growing season.

AGRONOMY JOURNAL (2021)

Article Chemistry, Multidisciplinary

Extraction of a Docosahexaenoic Acid-Rich Oil from Thraustochytrium sp. Using a Hydrophobic Ionic Liquid

Yujie Zhang, Valerie Ward, Samir Meramo, Dorothy Dennis, Natalia V. Plechkova, Roberto E. Armenta, Lars Rehmann

Summary: In this study, a novel hydrophobic ionic liquid (IL) was used as a pretreatment to aid in the extraction of DHA-rich oil from T18 biomass in the aqueous phase. The extraction conditions were optimized using a central composite design and response surface methodology, resulting in a high oil yield of 69.4% (w/w) and an extraction efficiency of 97.4%. This research demonstrates the efficient and sustainable recovery of DHA-rich oil from water using the proposed approach.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2023)

Article Engineering, Environmental

Assessment of the effects of biochar on biogas production during anaerobic digestion of aqueous pyrolysis condensate: A circular economy approach

Neha Batta, Tahereh Sarchami, Cesar M. Moreira, Lars Rehmann, Franco Berruti

Summary: The pyrolysis of biomass produces bio-oil, non-condensable gas, and biochar. This study focuses on utilizing the aqueous phase of the bio-oil, known as aqueous pyrolysis condensate (APC), for energy generation through anaerobic digestion with the presence of biochar derived from the digestate. The addition of biochar increased cumulative biogas production by 83% at the highest APC loading, demonstrating the potential of utilizing APC as a precursor for energy generation.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2023)

Article Chemistry, Multidisciplinary

Synthesis of FeO@SiO2-DNA core-shell engineered nanostructures for rapid adsorption of heavy metals in aqueous solutions

David Patino-Ruiz, Lars Rehmann, Mehrab Mehrvar, Edgar Quinones-Bolanos, Adriana Herrera

RSC ADVANCES (2020)

Article Biotechnology & Applied Microbiology

Increased Selectivity for Butanol in Clostridium Pasteurianum Fermentations via Butyric Acid Addition or Dual Feedstock Strategy

Garret Munch, Justus Mittler, Lars Rehmann

FERMENTATION-BASEL (2020)

Article Engineering, Environmental

Temperature-modulated sensing characteristics of ultrafine Au nanoparticle-loaded porous ZnO nanobelts for identification and determination of BTEX

Shun-Shun Chen, Xu-Xiu Chen, Tian-Yu Yang, Li Chen, Zheng Guo, Xing-Jiu Huang

Summary: A temperature-modulated sensing strategy was proposed to identify and determine BTEX compounds. Highly effective identification of BTEX was achieved using linear discrimination and convolutional neural network analyses. Additionally, quantitative analysis of concentration was accomplished by establishing the relationship between concentration and response.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Particulate matter-induced metabolic recoding of epigenetics in macrophages drives pathogenesis of chronic obstructive pulmonary disease

Myungkyung Noh, Jeong Yeon Sim, Jisung Kim, Jee Hwan Ahn, Hye-Young Min, Jong-Uk Lee, Jong-Sook Park, Ji Yun Jeong, Jae Young Lee, Shin Yup Lee, Hyo-Jong Lee, Choon-Sik Park, Ho-Young Lee

Summary: This study reveals that chronic exposure to PM induces chronic inflammation and development of COPD by dysregulating NAD+ metabolism and subsequent SIRT1 deficiency in pulmonary macrophages. Activation of SIRT1 by resveratrol effectively mitigates PM-induced inflammation and COPD development. Targeting metabolic and epigenetic reprogramming in macrophages induced by PM is a promising strategy for COPD treatment.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Electrocatalytic degradation of nitrogenous heterocycles on confined particle electrodes derived from ZIF-67

Yu Liu, Linlin Qin, Yiming Qin, Tong Yang, Haoran Lu, Yulong Liu, Qiqi Zhang, Wenyan Liang

Summary: Co/NC/PAC electrode was prepared by compounding ZIF-67 with powder-activated carbon for the electrocatalytic treatment of nitrogen-containing heterocyclic compounds. The degradation efficiency of the four compounds reached 90.2-93.7% under optimal conditions, and the degradation order was pyridazine < pyrimidine < pyrazine < pyridine.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Yttrium speciation variability in bauxite residues of various origins, ages and storage conditions

Julien Couturier, Pierre Tamba Oulare, Blanche Collin, Claire Lallemand, Isabelle Kieffer, Julien Longerey, Perrine Chaurand, Jerome Rose, Daniel Borschneck, Bernard Angeletti, Steven Criquet, Renaud Podor, Hamed Pourkhorsandi, Guilhem Arrachart, Clement Levard

Summary: This study analyzes the properties of bauxite residue samples and explores the influence of bauxite ore origin, storage conditions, and storage time. The results show that the speciation of yttrium is related to the origin of bauxite ore, while no significant variation was observed with storage conditions or aging of the residues.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Trophic transfer and their impact of microplastics on estuarine food chain model

Sakthinarenderan Saikumar, Ravi Mani, Mirunalini Ganesan, Inbakandan Dhinakarasamy, Thavamani Palanisami, Dharani Gopal

Summary: Microplastic contamination in marine ecosystems poses a growing concern due to its trophic transfer and negative effects on marine organisms. This study investigates the transfer and impacts of polystyrene microplastics in an estuarine food chain. The results show that microplastics can be transferred through the food chain, although the transfer rates are low. The exposed organisms exhibit stress responses, suggesting the potential risk of microplastics reaching humans through the food chain.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Review Engineering, Environmental

Antibiotic resistance genes and heavy metals in landfill: A review

Yan-Jiao Li, Ying Yuan, Wen-Bing Tan, Bei-Dou Xi, Hui Wang, Kun-Long Hui, Jia-Bao Chen, Yi-Fan Zhang, Lian-Feng Wang, Ren-Fei Li

Summary: This review investigated and analyzed the distribution, composition, and abundance of heavy metals and antibiotic resistance genes (ARGs) in landfill. The results showed that heavy metals have lasting effects on ARGs, and complexes of heavy metals and organic matter are common in landfill. This study provides a new basis to better understand the horizontal gene transfer (HGT) of ARGs in landfill.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

The effect of synthesis conditions on the in situ grown MIL-100(Fe)-chitosan beads: Interplay between structural properties and arsenic adsorption

Jessy Joseph, Ari Vaisanen, Ajay B. Patil, Manu Lahtinen

Summary: Efficient and environmentally friendly porous hybrid adsorbent beads have been developed for the removal of arsenic from drinking water. The structural tuning of the adsorbents has been shown to have a significant impact on their adsorption performance, with high crystallinity leading to increased adsorption capacity and selectivity towards As5+.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Phthalate metabolites in breast milk from mothers in Southern China: Occurrence, temporal trends, daily intake, and risk assessment

Yangyang Liu, Minhua Xiao, Kaiqin Huang, Juntao Cui, Hongli Liu, Yingxin Yu, Shengtao Ma, Xihong Liu, Meiqing Lin

Summary: This study measured the levels of phthalate metabolites in breast milk collected from mothers in southern China. The results showed that phthalates are still prevalent in the region, and breastfeeding contributes to phthalate intake in infants. However, the levels detected do not pose significant health risks to infants based on dietary exposure. The increasing exposure to certain phthalates calls for further research into their sources and potential risks.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Depth significantly affects plastisphere microbial evenness, assembly and co-occurrence pattern but not richness and composition

Zhiqiang Wu, Jianxing Sun, Liting Xu, Hongbo Zhou, Haina Cheng, Zhu Chen, Yuguang Wang, Jichao Yang

Summary: Ocean depth affects microbial diversity, composition, and co-occurrence patterns of microplastic microbial communities. Deterministic processes dominate the assembly of mesopelagic plastisphere microbial communities, while stochastic processes shape the assembly of bathypelagic microbial communities. The relationships between microorganisms in the mesopelagic layer are more complex and stable, with Proteobacteria and Actinobacteriota playing important roles.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Abatement of antibiotics and resistance genes during catalytic ozonation enhanced sludge dewatering process: Synchronized in volume and hazardousness reduction

Tingting Xiao, Renjie Chen, Chen Cai, Shijie Yuan, Xiaohu Dai, Bin Dong, Zuxin Xu

Summary: Based on the efficiency of catalytic ozonation techniques in enhancing sludge dewaterability, this study investigated its effectiveness in simultaneous reduction of antibiotics and antibiotic resistance genes. The results showed that catalytic ozonation conditioning changed the distribution of antibiotics and achieved high degradation rates. It also significantly reduced the abundance of ARGs, inhibited horizontal gene transfer, and decreased the signal transduction of typical ARGs host bacteria.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Unlocking the potential of ferrate(VI) in water treatment: Toward one-step multifunctional solutions

Yang Deng, Xiaohong Guan

Summary: This article discusses two different development approaches for ferrate(VI) technology in water treatment, arguing that process integration is a promising method that can drive technological innovation and revolution in water treatment, achieving higher treatment efficiency, reduced costs and energy consumption, and a smaller physical footprint.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Floating Catalytic Foam with prominent heat-induced convection for the effective photocatalytic removal of antibiotics

Zhe Zhang, Lu Zhang, Zhihao Huang, Yuxin Xu, Qingqing Zhao, Hongju Wang, Meiqing Shi, Xiangnan Li, Kai Jiang, Dapeng Wu

Summary: In this study, a floating catalytic foam was designed and prepared to enhance the mass transfer in immobilized photocatalysts for wastewater treatment. The floating catalytic foam could float on the water surface and establish a temperature gradient, effectively promoting the diffusion and adsorption of target molecules during the photocatalytic process.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Mechanism and synergistic effect of sulfadiazine (SDZ) and cadmium toxicity in spinach (Spinacia oleracea L.) and its alleviation through zinc fortification

Muhammad Nafees, Adiba Khan Sehrish, Sarah Owdah Alomrani, Linlin Qiu, Aasim Saeed, Shoaib Ahmad, Shafaqat Ali, Hongyan Guo

Summary: The accumulation of cadmium and antibiotics in edible plants and fertile soil is a worldwide problem. This study investigated the potential of zinc oxide nanoparticles to alleviate the toxicity of both cadmium and antibiotics and promote spinach growth.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Aminoalkyl organosilicon with dual chemical sites for SO2 absorption and analysis of site-specific absorption entropy and enthalpy

Lurui Wan, Kai Wang, Yuan Chen, Zhiyong Xu, Wenbo Zhao

Summary: In this study, a low viscosity and high thermal stability SO2 absorbent with dual interacting sites was successfully synthesized. The absorbent showed the highest absorption enthalpy change and entropy change values among reported SO2 absorbents, and exhibited lower viscosity and comparable thermal stability to ILs.

JOURNAL OF HAZARDOUS MATERIALS (2024)

Article Engineering, Environmental

Improvement of Fe(III)/percarbonate system by molybdenum powder and tripolyphosphate: Co-catalytic performance, low oxidant consumption, pH-dependent mechanism

Zhengwei Zhou, Guojie Ye, Yang Zong, Zhenyu Zhao, Deli Wu

Summary: This study utilized Mo powder and STPP to enhance the performance of the sodium percarbonate system in pollutant degradation. The presence of Mo and STPP resulted in a higher degradation rate of the model pollutant SMX, with low oxidant consumption. The system generated multiple active species through a series of chain reactions at different pH values, exhibiting excellent performance towards electron-rich pollutants. Furthermore, Mo demonstrated excellent stability and reusability.

JOURNAL OF HAZARDOUS MATERIALS (2024)