4.8 Article

Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state

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NATURE PHYSICS
卷 12, 期 2, 页码 150-156

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NATURE PUBLISHING GROUP
DOI: 10.1038/NPHYS3519

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资金

  1. Center for Emergent Superconductivity, an Energy Frontier Research Center at Brookhaven National Laboratory
  2. US Department of Energy [DE-2009-BNL-PM015]
  3. Ministry of Science and Education (Japan)
  4. Global Centers of Excellence Program for Japan Society for the Promotion of Science
  5. FlucTeam Program at Brookhaven National Laboratory [DE-AC02-98CH10886]
  6. EPSRC through Programme Grant 'Topological Protection and Non-Equilibrium States in Correlated Electron Systems'
  7. US Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-SC0010313]
  8. NSF [DMR-1103860]
  9. Templeton Foundation
  10. Government of Canada through Industry Canada
  11. Province of Ontario through Ministry of Research and Innovation
  12. Direct For Mathematical & Physical Scien
  13. Division Of Materials Research [1360789] Funding Source: National Science Foundation
  14. Engineering and Physical Sciences Research Council [1265368, EP/I031014/1] Funding Source: researchfish
  15. EPSRC [EP/I031014/1] Funding Source: UKRI

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Research on high-temperature superconducting cuprates is at present focused on identifying the relationship between the classic ` pseudogap' phenomenon(1,2) and the more recently investigated density wave state(3-13). This state is generally characterized by a wavevector Q parallel to the planar Cu-O-Cu bonds(4-13) along with a predominantly d-symmetry form factor(14-16) (dFF-DW). To identify the microscopic mechanism giving rise to this state(17-29), one must identify the momentum-space states contributing to the dFF-DW spectral weight, determine their particle-hole phase relationship about the Fermi energy, establish whether they exhibit a characteristic energy gap, and understand the evolution of all these phenomena throughout the phase diagram. Here we use energy-resolved sublattice visualization(14) of electronic structure and reveal that the characteristic energy of the dFF-DW modulations is actually the 'pseudogap' energy Delta 1. Moreover, we demonstrate that the dFF-DW modulations at E = -Delta(1) (filled states) occur with relative phaseffcompared to those at E = -Delta(1) (empty states). Finally, we show that the conventionally defined dFF-DW Q corresponds to scattering between the ` hot frontier' regions of momentum-space beyond which Bogoliubov quasiparticles cease to exist(30-32). These data indicate that the cuprate dFF-DW state involves particle-hole interactions focused at the pseudogap energy scale and between the four pairs of ` hot frontier' regions in momentum space where the pseudogap opens.

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