Article
Polymer Science
Sotirios Kopsidas, Ganiu B. Olowojoba, Chris Stone, David Clark, A. Manu Haddad, Anthony J. Kinloch, Ambrose C. Taylor
Summary: In this study, the electrical conductivity of carbon-fiber reinforced polymer (CFRP) composites was improved by adding graphene nanoplatelets (GNPs) and carbon nanotubes (CNTs). The modified CFRP laminates demonstrated superior electrical performance and resistance against lightning strike damage, while reducing weight by 20%.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Polymer Science
Jefersson Alexander Rojas, Luis Felipe de Paula Santos, Edson Cocchieri Botelho, Bruno Ribeiro, Mirabel Cerqueira Rezende
Summary: Combining multi-walled carbon nanotube buckypapers with glass fiber/epoxy resin composites can achieve good electromagnetic interference shielding effectiveness in the X-band and Ku-band; however, adding CNT film to the composites did not improve the elastic properties but rather decreased compression shear and interlaminar shear strength.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Polymer Science
Salman Mahaki, Hamed Khosravi, Esmaeil Tohidlou
Summary: In this study, a chemical precipitation method was used to decorate graphene oxide (GO) with Fe2O3 nanoparticles, resulting in improved mechanical properties of epoxy (EP) composites. Specifically, the hybrid composites containing 0.2 and 0.6 wt% Fe2O3@GO showed the best flexural and wear behaviors.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Polymer Science
Noorshashillawati Azura Mohammad, Sahrim Hj Ahmad, Ruey Shan Chen, Nurul Emi Nor Ain Mohammad
Summary: The introduction of graphene nanoplatelets into rubber toughened epoxy matrix showed significant enhancement in mechanical and thermal properties. The incorporation of GNP optimized tensile strength and modulus, while also improving thermal stability and interfacial interaction between matrix and nanofiller. XRD analysis confirmed the dispersion states of GNP in the epoxy/LENR, highlighting the potential of GNP in enhancing composites.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Polymer Science
Abhishek K. Pathak, Lekha Sharma, Hema Garg, Tomohiro Yokozeki, Sanjay R. Dhakate
Summary: In situ chemical linkage between amine-functionalized graphene and epoxy polymer has been successfully achieved, leading to improved mechanical and thermal properties of nanocomposites. The formation of a chemical bond between the graphene and epoxy is demonstrated and its mechanism is derived based on experimental evidence.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Polymer Science
Sotirios Kopsidas, Ganiu B. Olowojoba
Summary: Epoxy polymers were modified with a hybrid nanofiller containing graphene nanoplatelets (GNPs) and carbon nanotubes (CNTs) at a mass ratio of 9:1, resulting in a significant increase in electrical conductivity and fracture energy. The reduced percolation threshold was attributed to CNTs, while the increased toughness was mainly due to GNPs through crack deflection. The toughening contribution of the hybrid nanofiller was accurately predicted using analytical modeling.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Qi Qin, Jing Chen, Changze Wu, Yixue Wang, Yunan Li, Meng Song
Summary: Novel carbon nanostructures, carbon nanobuds and nanoballs, have been successfully synthesized on the surface of graphene using the electrochemical method. Under a certain potential, carbon nanobuds are grown in situ on the surface of graphene, and with the increase of potential, these nanobuds grow into nanoballs and exfoliate from the graphene surface. Graphene undergoes oxidation at higher potentials, resulting in the formation of graphene oxide fragments.
Article
Polymer Science
Ana Carolina Prataviera Sarturato, Erick Gabriel Ribeiro Dos Anjos, Juliano Marini, Guilherme Ferreira De Melo Morgado, Mauricio Ribeiro Baldan, Fabio Roberto Passador
Summary: Polypropylene (PP)/talc composites are widely used in various industries, but the demand for more efficient and environmentally friendly materials is increasing, leading to the exploration of new reinforcements. Graphene nanoplates (GNP) offer a good alternative due to their ability to enhance properties and optimize processes. This study investigated the effects of adding different weight percentages of GNP to PP/talc composites and found that it led to improvements in various properties such as flow behavior, mechanical strength, and electrical conductivity.
JOURNAL OF APPLIED POLYMER SCIENCE
(2023)
Article
Polymer Science
Qiao Li, Guangyi Lin, Shouzhen Chen, Lin Zhang, Yingjie Song, Chuanbao Geng, Siyuan Qu, Yuan Jing, Fumin Liu, Zhenning Liang
Summary: This study focused on the wet skid resistance and thermal conductivity of green tires. By grafting amino and epoxy groups onto the surface of SiO2 and graphene oxide (GO) using different types of silane coupling agents, the researchers were able to improve the performance of rubber composites. The hybrid filler, containing amino and epoxy groups, not only enhanced the interface compatibility and synergistic reinforcement effect, but also resulted in excellent wet skid resistance and mechanical properties.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Polymer Science
Zhuyi Gao, Qunfeng Dong, Mengyao Shang, Baoqing Shentu, Chinan Wu
Summary: This study investigated the effects of CNTs/GNPs hybrid fillers on the properties of PBT/PET composites prepared by melt blending process. The hybrid fillers were found to enhance mechanical properties and thermal conductivity, as well as improve electrical conductivity and EMI SE. Absorption loss was identified as the main mechanism for the attenuation of incident electromagnetic waves in the hybrid composites.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Review
Polymer Science
Euphrasie Jasinski, Veronique Bounor-Legare, Aurelie Taguet, Emmanuel Beyou
Summary: The study investigates the influence of halloysite nanotubes as carriers of flame retardant systems on the fire retardancy performances of polymer-based composites, aiming for long-term aging properties.
POLYMER DEGRADATION AND STABILITY
(2021)
Article
Polymer Science
Camila Mouta Caldas, Bluma Guenther Soares, Tamara Indrusiak, Guilherme Mariz Oliveira Barra
Summary: By modifying PMMA nanocomposites and incorporating GNP with different fluorinated ionic liquids, composites with high thermal stability and conductivity can be obtained, showing excellent absorption properties in terms of microwave absorption.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Polymer Science
Pavan Kumar Gangineni, Satyaroop Patnaik, Rajesh Kumar Prusty, Bankim Chandra Ray
Summary: The study showed that modifying carbon fiber reinforced polymer (CFRP) composites with graphene carboxyl can improve mechanical properties at elevated temperatures, but may lead to reduced strength under high temperature conditions compared to neat composites.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Polymer Science
Xiaoling Luo, Dirk W. Schubert
Summary: This study fabricated PMMA/GNPs conductive composite films with different morphologies using four fabrication techniques and systematically investigated the morphologies of dispersed GNPs and their electrical properties in both in-plane and perpendicular direction. The percolation thresholds and conductivities of the composites varied significantly with different fabrication techniques, and the differences were explained in terms of GNPs size, orientation, distribution, and dispersion state.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Polymer Science
Li Chen, Xiujiang Pang, Yi Kang
Summary: Both graphene and carbon nanotubes can improve the crosslinking density, reduce rolling resistance, and wet-skid resistance of NR composites. Compared to CNTs, graphene degrades manufacturing safety and cure rate, but exhibits a higher reinforcing effect in terms of tensile strength, modulus, and hardness. Additionally, graphene/NR composites show better aging resistance than CNTs/NR. On the other hand, CNTs can improve manufacturing safety and cure rate, maintain higher tear strength, and provide better tensile fatigue and wear resistance, as well as lowering rolling resistance while maintaining higher wet-skid resistance in comparison to graphene.
JOURNAL OF APPLIED POLYMER SCIENCE
(2022)
Article
Engineering, Environmental
Kangqi Chang, Minhao Guo, Lei Pu, Jiancheng Dong, Le Li, Piming Ma, Yunpeng Huang, Tianxi Liu
Summary: Researchers have developed a hybrid nanofibrous tactile sensor that exhibits high sensitivity and superior stability, making it promising for applications in electronic skin and human-machine interfaces. The sensor demonstrates a wide working range, rapid response/recovery times, and long-term durability, and can be assembled into a wearable wireless sensor for real-time detection of human activity signals.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Materials Science, Multidisciplinary
Guanglong Li, Jing Huang, Xuhui Zhang, Yang Wang, Jinliang Qiao, Tianxi Liu, Mingliang Du, Weifu Dong
Summary: This study reports sustainable thermosets based on dynamic acylhydrazone bonds made from biomass acid derivatives. These thermosets have renewable raw materials, can be recycled to maintain mechanical properties, and have reduced use of organic solvents during material preparation and recycling. Additionally, they exhibit excellent mechanical performance and heat resistance. The acylhydrazone bonds in the thermoset networks enhance hydrophobicity and water resistance. Overall, these thermosets provide a solution for developing sustainable materials.
MACROMOLECULAR MATERIALS AND ENGINEERING
(2023)
Article
Polymer Science
Xiang Chen, Chenxi Hu, Yang Wang, Ting Li, Jie Jiang, Jing Huang, Shibo Wang, Tianxi Liu, Weifu Dong, Jinliang Qiao
Summary: This study systematically investigates the optical properties of poly(maleic anhydride-alt-vinyl acetate) (PMV) synthesized using different polymerization methods. It is found that solution polymerization and redissolving methods can increase the quantum yield of the polymer. The study also suggests that good solvents can reduce the rigidity of the polymer chains and promote the formation of clusters.
MACROMOLECULAR RAPID COMMUNICATIONS
(2023)
Article
Chemistry, Physical
Xinwei Tang, Jiangtao Luo, Zhiwei Hu, Shijie Lu, Xiaoyi Liu, Shuangshuang Li, Xu Zhao, Zihang Zhang, Qianqian Lan, Piming Ma, Zicheng Wang, Tianxi Liu
Summary: In this study, a novel MXene-based graphene porous film with ultrathin, flexible, and oxidation-resistant characteristics was successfully fabricated. The porous conductive network in the film efficiently shields electromagnetic waves, achieving excellent shielding performance. Moreover, the film exhibits durability and maintains high shielding performance for up to 12 months.
Article
Chemistry, Multidisciplinary
Yeshu Tan, Jianrui Feng, Haobo Dong, Longxiang Liu, Siyu Zhao, Feili Lai, Tianxi Liu, Ying Bai, Ivan P. Parkin, Guanjie He
Summary: This study fabricates unique heterostructures by depositing platinum nanocrystals on the edge of transition metal phosphide nanosheets, showing outstanding HER performance in an alkaline medium. The heterostructures exhibit low platinum usage amount and excellent stability. Additionally, the study provides a new strategy for designing enhanced HER performance.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Hanjun Li, Honggang Huang, Yao Chen, Feili Lai, Hui Fu, Longsheng Zhang, Nan Zhang, Shuxing Bai, Tianxi Liu
Summary: High-entropy alloy aerogels (HEAAs) show great potential as new catalysts for the carbon dioxide reduction reaction (CO2RR). The PdCuAuAgBiIn HEAAs fabricated using the freeze-thaw method exhibit almost 100% Faradaic efficiency for C1 products and outperform other materials, thanks to the strong interactions between different metals and the regulation of unsaturated surface sites.
ADVANCED MATERIALS
(2023)
Article
Engineering, Environmental
Le Li, Yufeng Wang, Xuran Bao, Dai Hai Nguyen, Chao Zhang, Tianxi Liu
Summary: This study presents the fabrication of a host-guest hybrid gel electrode composed of poly-pyrrole aerogel and Fe-PAA hydrogel. The electrode exhibits high elasticity and self-healing properties, making it suitable for all-gel-state supercapacitors with thickness-independent capacitive performance. The interfacial polymerization approach is used to prepare the pseudocapacitive PPy aerogel as a host component, and the ionically conductive and self-healable Fe-PAA hydrogel as a guest component, resulting in enhanced electron/ion transport kinetics and thickness-independent supercapacitance.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Multidisciplinary
Qiaoran Zhang, Lei Ma, Tiantian Xue, Jing Tian, Wei Fan, Tianxi Liu
Summary: This study introduces a novel double-layer smart textile made of polyimide aerogel fiber, which combines excellent fire resistance with thermal regulation. The outer layer reduces peak heat release rate, exhibiting outstanding fire resistance, while the inner layer delays temperature rise during phase change, providing cool somatosensory temperature for firefighters. The double-layer textile extends the time to pain threshold of human skin, showing great potential for next-generation firefighting clothing.
COMPOSITES PART B-ENGINEERING
(2023)
Article
Materials Science, Multidisciplinary
Shuangshuang Li, Xinwei Tang, Xu Zhao, Shijie Lu, Jiangtao Luo, Zheyuan Chai, Tiantian Ma, Qianqian Lan, Piming Ma, Weifu Dong, Zicheng Wang, Tianxi Liu
Summary: In this study, an ultralight magnetic composite foam with hierarchical impedance structure was developed by electrostatic self-assembly of MXene on graphene skeletons and subsequent hydrothermal anchoring of FeS clusters. The composite foam exhibited high microwave absorption performance, with a minimum reflection loss of -47.17 dB and an effective absorption bandwidth of 6.15 GHz at a thickness of 4.78 mm. The microwave absorption performance of the foam could be further optimized by controlling the loading of MXene and applying low-temperature thermal treatment.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2023)
Article
Chemistry, Multidisciplinary
Hui Zheng, Yizhe Zhang, Yang Wang, Zhenzhong Wu, Feili Lai, Guojie Chao, Nan Zhang, Longsheng Zhang, Tianxi Liu
Summary: Electrochemical nitrate reduction to ammonia (NRA) is an efficient and sustainable method to convert nitrate pollutants into value-added products. Research has shown that the amount of oxygen vacancies in perovskite oxides is related to their catalytic activity towards NRA.
Article
Chemistry, Physical
Xiao Yao, Jin Wang, Shiru Lin, Chengzhou Tao, Xuezhi Zhang, Wei Wang, Chengcheng Zhao, Lina Wang, Junwei Lucas Bao, Yonggang Wang, Tianxi Liu
Summary: This study proposes a method of stabilizing the solid-electrolyte interphase (SEI) of lithium-metal batteries through sodium bromination treatment, and investigates the mechanism of sodium bromide in inhibiting dendritic lithium growth. The results show that incorporating sodium bromide into the SEI ensures the cycling stability of lithium-metal batteries under different conditions, with extended lifespan and good rate capability.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Jingyi Wang, Jianrui Feng, Yuying Li, Feili Lai, Gui-Chang Wang, Tianxi Liu, Jiajia Huang, Guanjie He
Summary: In this study, a novel structure of self-supported electrocatalyst Co-ALMO@NF was synthesized using a hydrothermal method. The Co-ALMO@NF exhibited excellent electrocatalytic performances, requiring low voltage and achieving high current density. The structural design of self-supported electrocatalysts was highlighted as important.
Article
Chemistry, Multidisciplinary
Wen-Ya Wu, Sida Wu, Weng Weei Tjiu, Hui Ru Tan, Fong Yew Leong, Poh Chong Lim, Suxi Wang, Wenbin Jiang, Rong Ji, Qiang Zhu, Michel Bosman, Qingyu Yan, Zainul Aabdin
Summary: This study reports the synthesis of Ag/Pt and Ag/Pd core/shell nanocrystals and provides insights into the formation mechanism of these bimetallic core/shell nanocrystals during oxygen plasma treatment. The findings deepen our understanding of the interface dynamics of bimetallic nanostructured catalysts under an oxidative environment and reveal an alternative approach for catalyst pretreatment.
Article
Chemistry, Physical
Xiaohui Yu, Yufei Wang, Haopeng Zhang, Zibiao Li, Yong Zheng, Xiaoshan Fan, Yan Lv, Xu Zhang, Tianxi Liu
Summary: A facile strategy for fabricating high-performance hydrogels with strain-stiffening behavior, self-healing ability, and low hysteresis is proposed. The unique structure of the hydrogels, which consists of two mechanically distinct polymeric networks, gives them unique properties suitable for applications such as strain sensors and human motion detection.
CHEMISTRY OF MATERIALS
(2023)
Article
Chemistry, Physical
Yufan Huang, Xu Zhang, Tianyi Zhu, Yufeng Wang, Nan Hu, Zeyu Ren, Xiaohui Yu, Dai Hai Nguyen, Chao Zhang, Tianxi Liu
Summary: A salting-out bioriented nanocomposite hydrogel (s-BNCH) with high mechanical strength and superior stretchability has been developed through a reactive freeze-casting procedure. The s-BNCH exhibits anisotropic mechanical properties and ionic conductivity, making it suitable for skin-inspired sensors with impressive strain-sensing performance and puncture resistance.
CHEMISTRY OF MATERIALS
(2023)