期刊
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL
卷 5, 期 6, 页码 1489-1497出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.ijggc.2011.08.006
关键词
CFD modeling; CFB; Oxy-coal combustion; Desulfurization
类别
资金
- National Key Program of Basic Research of China [2006CB705806, 2011CB707301]
- State Key Laboratory of Coal Combustion [FSKLCC1006]
Based on the Computational Fluid Dynamics (CFD) method, the previously established and validated 2-dimensional model was employed to predict the oxy-coal combustion processes in a 50 kW circulating fluidized bed (CFB) at Southeast University, China. The simulated processes of coal conversion in our CFB combustion system included particle drying, dry coal devolatilization, volatile combustion, char combustion, char gasification and SO2 emission. The effects of combustion atmospheres, including air (21% O-2/79% N-2) and oxygen/recycled flue gas (O-2/RFG) atmosphere with different O-2 concentration (from 21% to 40%), were investigated on distributions of solid volume fraction, temperature and gas concentration in the riser. During combustion of Xuzhou bituminous coal in O-2/RFG modes with different O-2 concentrations referred to above, about 70% volume fraction of CO2 were achieved in the wet flue gas with more than 25% volume fraction of H2O. The rates of char gasification by CO2 and H2O in 30% O-2/70% RFG atmosphere were obviously higher than that in air. However, compared to air combustion, CO concentration in the dense zone in 30% O-2/70% RFG atmosphere was lower because high concentration of H2O accelerated CO combustion. Both indirect and direct desulfurization mechanisms were considered for sulfur retention by limestone and the corresponding overall reaction rates were calculated statistically. With increase in O-2 inlet concentration gaseous pollutant SO2 was enriched. (C) 2011 Elsevier Ltd. All rights reserved.
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