期刊
INORGANIC CHEMISTRY
卷 51, 期 15, 页码 8538-8544出版社
AMER CHEMICAL SOC
DOI: 10.1021/ic301115b
关键词
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资金
- NSFC [91122032, 90922009, 21121061]
- 973 Project [2012CB821704]
- K. U. Leuven
- ANR-PNANO [ANR-08-NANO-002]
- ERC [226558]
The field-induced blockage of magnetization behavior was first observed in an Yb-III-based molecule with a trigonally distorted octahedral coordination environment. Ab initio calculations and micro-SQUID measurements were performed to demonstrate the exhibition of easy-plane anisotropy, suggesting the investigated complex is the first pure lanthanide field-induced single-ion magnet (field-induced SIM) of this type. Furthermore, we found the relaxation time obeys a power law instead of an exponential law, indicating that the relaxation process should be involved a direct process rather than an Orbach process.
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