☆ 4.7 Article

Crystalline-state guest-exchange and gas-adsorption phenomenon for a Soft supramolecular porous framework stacking by a rigid linear coordination polymer

INORGANIC CHEMISTRY (2008)

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INORGANIC CHEMISTRY

卷 47, 期 12, 页码 5218-5224

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AMER CHEMICAL SOC

DOI: 10.1021/ic800050u

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Chemistry, Inorganic & Nuclear

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A 1D rigid, linear coordination polymer, (4,4 '-bipyridine)(2-pyridylsulfonate)copper, has been applied for the controlled-assembly of a new porous host that generates 1D channels by an interdigitated packing through the recognition of hydrogen bonding and pi-pi stacking interactions. The porous structure is architecturally robust when it reversibly uptakes water molecules and exchanges guest small molecules (MeOH, i-PrOH) from solution as determined by single-crystal-to-single-crystal transformation studies. Moreover, the open-channel solid displays irreversible benzene and toluene vapor sorption behaviors attributed to a widening of the channel cross-section that fetters the larger guest molecules, resulting from the dynamic, soft supramolecular framework.

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Ossowska, J. M. Otalora Goicochea, T. Ovsiannikova, P. Owen, A. Oyanguren, B. Pagare, P. R. Pais, T. Pajero, A. Palano, M. Palutan, Y. Pan, G. Panshin, A. Papanestis, M. Pappagallo, L. L. Pappalardo, C. Pappenheimer, W. Parker, C. Parkes, C. J. Parkinson, B. Passalacqua, G. Passaleva, A. Pastore, M. Patel, C. Patrignani, C. J. Pawley, A. Pearce, A. Pellegrino, M. Pepe Altarelli, S. Perazzini, D. Pereima, P. Perret, M. Petric, K. Petridis, A. Petrolini, A. Petrov, S. Petrucci, M. Petruzzo, T. T. H. Pham, A. Philippov, L. Pica, M. Piccini, B. Pietrzyk, G. Pietrzyk, M. Pili, D. Pinci, F. Pisani, P. K. Resmi, V Placinta, J. Plews, M. Plo Casasus, F. Polci, M. Poli Lener, M. Poliakova, A. Poluektov, N. Polukhina, I Polyakov, E. Polycarpo, G. J. Pomery, S. Ponce, D. Popov, S. Popov, S. Poslavskii, K. Prasanth, L. Promberger, C. Prouve, V Pugatch, H. Pullen, G. Punzi, W. Qian, J. Qin, R. Quagliani, B. Quintana, N. Raab, R. I. Rabadan Trejo, B. Rachwal, J. H. Rademacker, M. Rama, M. 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Shapkin, I Shchemerov, L. Shchutska, T. Shears, L. Shekhtman, Z. Shen, V Shevchenko, E. B. Shields, E. Shmanin, J. D. Shupperd, B. G. Siddi, R. Silva Coutinho, G. Simi, S. Simone, N. Skidmore, T. Skwarnicki, M. W. Slater, I Slazyk, J. C. Smallwood, J. G. Smeaton, A. Smetkina, E. Smith, M. Smith, A. Snoch, M. Soares, L. Soares Lavra, M. D. Sokoloff, F. J. P. Soler, A. Solovev, I Solovyev, F. L. Souza De Almeida, B. Souza De Paula, B. Spaan, E. Spadaro Norella, P. Spradlin, F. Stagni, M. Stahl, S. Stahl, P. Stefko, O. Steinkamp, O. Stenyakin, H. Stevens, S. Stone, M. E. Stramaglia, M. Straticiuc, D. Strekalina, F. Suljik, J. Sun, L. Sun, Y. Sun, P. Svihra, P. N. Swallow, K. Swientek, A. Szabelski, T. Szumlak, M. Szymanski, S. Taneja, F. Teubert, E. Thomas, K. A. Thomson, V Tisserand, S. T'Jampens, M. Tobin, L. Tomassetti, D. Torres Machado, D. Y. Tou, M. T. Tran, E. Trifonova, C. Trippl, G. Tuci, A. Tully, N. Tuning, A. Ukleja, D. J. Unverzagt, E. Ursov, A. Usachov, A. Ustyuzhanin, U. Uwer, A. Vagner, V. Vagnoni, A. Valassi, G. Valenti, N. Valls Canudas, M. van Beuzekom, M. Van Dijk, E. van Herwijnen, C. B. Van Hulse, M. van Veghel, R. Vazquez Gomez, P. Vazquez Regueiro, C. Vazquez Sierra, S. Vecchi, J. J. Velthuis, M. Veltri, A. Venkateswaran, M. Veronesi, M. Vesterinen, D. Vieira, M. Vieites Diaz, H. Viemann, X. Vilasis-Cardona, E. Vilella Figueras, P. Vincent, D. Vom Bruch, A. Vorobyev, V. Vorobyev, N. Voropaev, R. Waldi, J. Walsh, C. Wang, J. Wang, J. Wang, J. Wang, J. Wang, M. Wang, R. Wang, Y. Wang, Z. Wang, Z. Wang, H. M. Wark, N. K. Watson, S. G. Weber, D. Websdale, C. Weisser, B. D. C. Westhenry, D. J. White, M. Whitehead, D. Wiedner, G. Wilkinson, M. Wilkinson, I Williams, M. Williams, M. R. J. Williams, F. F. Wilson, W. Wislicki, M. Witek, L. Witola, G. Wormser, S. A. Wotton, H. Wu, K. Wyllie, Z. Xiang, D. Xiao, Y. Xie, A. Xu, J. Xu, L. Xu, M. Xu, Q. Xu, Z. Xu, Z. Xu, D. Yang, S. Yang, Y. Yang, Z. Yang, Z. Yang, Y. Yao, L. E. Yeomans, H. Yin, J. Yu, X. Yuan, O. Yushchenko, E. Zaffaroni, M. Zavertyaev, M. Zdybal, O. Zenaiev, M. Zeng, D. Zhang, L. Zhang, S. Zhang, Y. Zhang, Y. Zhang, A. Zhelezov, Y. Zheng, X. Zhou, Y. Zhou, X. Zhu, Z. Zhu, V Zhukov, J. B. Zonneveld, Q. Zou, S. Zucchelli, D. Zuliani, G. Zunica

Summary: In this study, the oscillation frequency of mesons composed of beauty and strange quarks was measured using B-s(0) -> D-s(-)pi(+) decays produced in proton-proton collisions at the LHCb detector. The measurement improved the precision of Delta m(s) by a factor of two compared to previous results when combined with other LHCb measurements.

NATURE PHYSICS (2022)

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Article Instruments & Instrumentation

Optimization of Timepix3-based conventional Compton camera using electron track algorithm

Jiaxing Wen, Xutao Zheng, Huaizhong Gao, Ming Zeng, Yuge Zhang, Minghai Yu, Yuchi Wu, Jirong Cang, Ge Ma, Zongqing Zhao

Summary: In this study, an electron track algorithm was used to improve the angular resolution of a single layer Compton camera based on Timepix3, enhancing the accuracy to 12 degrees. The method showed significant results in the experimental demonstration.

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (2022)

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Article Cell Biology

A novel long-term intravenous combined with local treatment with human amnion-derived mesenchymal stem cells for a multidisciplinary rescued uremic calciphylaxis patient and the underlying mechanism

Lianju Qin, Jing Zhang, Yujie Xiao, Kang Liu, Yugui Cui, Fangyan Xu, Wenkai Ren, Yanggang Yuan, Chunyan Jiang, Song Ning, Xiaoxue Ye, Ming Zeng, Hanyang Qian, Anning Bian, Fan Li, Guang Yang, Shaowen Tang, Zhihong Zhang, Juncheng Dai, Jing Guo, Qiang Wang, Bin Sun, Yifei Ge, Chun Ouyang, Xueqiang Xu, Jing Wang, Yaoyu Huang, Hongqing Cui, Jing Zhou, Meilian Wang, Zhonglan Su, Yan Lu, Di Wu, Jingping Shi, Wei Liu, Li Dong, Yinbing Pan, Baiqiao Zhao, Ying Cui, Xueyan Gao, Zhanhui Gao, Xiang Ma, Aiqin Chen, Jie Wang, Meng Cao, Qian Cui, Li Chen, Feng Chen, Youjia Yu, Qiang Ji, Zhiwei Zhang, Mufeng Gu, Xiaojun Zhuang, Xiaolin Lv, Hui Wang, Yanyan Pan, Ling Wang, Xianrong Xu, Jing Zhao, Xiuqin Wang, Cuiping Liu, Ningxia Liang, Changying Xing, Jiayin Liu, Ningning Wang

Summary: This study reported a case of severe uremic calciphylaxis patient who showed significant improvement after receiving treatment with human amnion-derived mesenchymal stem cells (hAMSCs). The long-term intravenous combined with local treatment of hAMSCs may be a potential regenerative treatment for uremic calciphylaxis.

JOURNAL OF MOLECULAR CELL BIOLOGY (2022)

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Article Food Science & Technology

The relationship between the formation of advanced glycation end products and quality attributes of fried sturgeon fillets

Qinyi Liu, Sheng Wang, Xueyang Wang, Shiyuan Dong, Yuanhui Zhao, Mingyong Zeng

Summary: This study investigated the effects of frying temperature and time on the formation of advanced glycation end products (AGEs) in fried fish. The results showed that frying time significantly increased the production of fluorescent-AGEs, while shorter frying times had less impact on the formation of specific AGEs. Correlation analysis revealed associations between fluorescent-AGEs and moisture and L*, CML and lipid content, and CEL and free sulfhydryl groups. The formation of AGEs was found to be less affected by oxidation. Based on principal component analysis, it was recommended to fry sturgeon fillets for 5 minutes at 170 or 180 degrees Celsius.

LWT-FOOD SCIENCE AND TECHNOLOGY (2022)

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Article Instruments & Instrumentation

206,207,208,natPb(p,x)194Hg and 209Bi(p,x)194Hg excitation functions in the energy range 0.04-2.6 GeV

Yu E. Titarenko, V. F. Batyaev, K. Pavlov, A. Yu Titarenko, S. Malinovskiy, V. Rogov, V. M. Zhivun, T. Kulevoy, M. Chauzova, R. S. Khalikov, A. Ignatyuk, V. Yu Blandinskiy, A. A. Kovalishin, M. Baznat, A. Yu Stankovskiy, A. Dubrouski, H. Kiyavitskaya, Tao Xue, Yang Tian, Ming Zeng, Zhi Zeng, O. Normahmedov, Tatsihiko Sato

Summary: This article presents the excitation results of Hg-194 in lead-bismuth eutectic on lead and bismuth isotopes in deep spallation reactions. The experimental data is compared with data from other authors and simulated using different high-energy transport codes and data libraries.

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (2022)

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Article Immunology

Evaluation of a recombinant five-antigen Staphylococcus aureus vaccine: The randomized, single-centre phase 1a/1b clinical trials

Feng-Cai Zhu, Hao Zeng, Jing-Xin Li, Bin Wang, Fan-Yue Meng, Feng Yang, Jiang Gu, Hao-Yu Liang, Yue-Mei Hu, Pei Liu, Liu-Sheng Peng, Xiao-Kui Hu, Yuan Zhuang, Min Fan, Hai-Bo Li, Zhong-Ming Tan, Ping Luo, Peng Zhang, Kai Chu, Jin-Yong Zhang, Ming Zeng, Quan-Ming Zou

Summary: This study evaluated the safety and immunogenicity of a recombinant five-antigen Staphylococcus aureus vaccine in healthy adults. The vaccine was found to be safe and well-tolerated, and it elicited strong humoral and cellular immune responses. Further research and development of this vaccine are warranted.

VACCINE (2022)

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Article Nutrition & Dietetics

Formation of Nε-Carboxymethyl-Lysine and Nε-Carboxyethyl-Lysine in Pacific Oyster (Crassostrea gigas) Induced by Thermal Processing Methods

Pengcheng Zhou, Shiyuan Dong, Mingyong Zeng

Summary: This study investigated the effects of different thermal processing methods on the formation of AGEs in Pacific oysters and found that sous vide treatment at 70 degrees C was effective in reducing AGEs formation. The levels of fat content, oxidation, and moisture content were found to have an impact on AGEs formation.

FRONTIERS IN NUTRITION (2022)

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Article Pediatrics

Short stature and melanocytic nevi in a girl with ARID1B-related Coffin-Siris syndrome: a case report

Dong-Ying Tao, Huan-Hong Niu, Jing-Jing Zhang, Hui-Qin Zhang, Ming-Hua Zeng, Sheng-Quan Cheng

Summary: This case report describes a girl with Coffin-Siris syndrome who presented with intellectual disability, short stature, and prominent cutaneous features. Whole exome sequencing identified a novel variant in the ARID1B gene. Treatment with recombinant human growth hormone resulted in significant improvement in height, and no enlargement or malignant transformation of nevi was observed during follow-up.

BMC PEDIATRICS (2022)

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Article Chemistry, Physical

Pt1/Ni6Co1 layered double hydroxides/N-doped graphene for electrochemical non-enzymatic glucose sensing by synergistic enhancement of single atoms and doping

Baojun Long, Peiyu Cao, Yuanmeng Zhao, Qianqian Fu, Yan Mo, Yueming Zhai, Juejing Liu, Xingyi Lyu, Tao Li, Xiaofeng Guo, Changsheng Shan, Minghua Zeng

Summary: This study reports a novel Pt single-atom catalyst for highly efficient electrochemical catalysis and sensing of glucose. The loading of Pt single atoms increases with Co doping, providing more anchoring sites for Pt SAs. The resulting Pt-1/Ni(6)Co(1)LDHs/NG exhibits low oxidative potential, high sensitivity, excellent selectivity, and great stability. The boosted performance of Pt-1/Ni(6)Co(1)LDHs/NG originates from its stronger binding energy with glucose and the synergistic effect of Pt SAs, Co doping, and NG.

NANO RESEARCH (2023)

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Article Chemistry, Applied

Novel Pickering emulsion stabilized by natural fiber polysaccharide-protein extracted from Haematococcus pluvialis residues

Zihao Yin, Mengwei Wang, Mingyong Zeng

Summary: In this study, aqueous protein extraction from H. pluvialis residues (APHRs) was successfully extracted, which had high content of protein and carbohydrate. APHRs showed excellent emulsifying stability and oil holding capacity, and microscopic observation revealed the presence of fibrous polysaccharides that formed stable structural cross-linking around protein particles. Compared to other residues, APHRs formed emulsions with the smallest particle size and best storage stability.

FOOD HYDROCOLLOIDS (2023)

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Article Plant Sciences

MtEIN2 affects nitrate uptake and accumulation of photosynthetic pigments under phosphate and nitrate deficiency in Medicago truncatula

Ming Zeng, Nicole M. van Dam, Bettina Hause

Summary: Ethylene (ET) controls various aspects of plant growth and development under both abiotic and biotic stresses. MtEIN2, a critical element in the ET signaling pathway, plays an important role in biotic interactions. However, its role in responding to abiotic stress, such as nutrient deficiency, is less understood.

PHYSIOLOGIA PLANTARUM (2023)

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Article Astronomy & Astrophysics

Search for exotic interactions of solar neutrinos in the CDEX-10 experiment

X. P. Geng, L. T. Yang, Q. Yue, K. J. Kang, Y. J. Li, H. P. An, C. Greeshma, J. P. Chang, Y. H. Chen, J. P. Chang, W. H. Dai, Z. Deng, C. H. Fang, H. Gong, Q. J. Guo, X. Y. Guo, L. He, S. M. He, J. W. Hu, H. X. Huang, T. C. Huang, H. T. Jia, X. Jiang, S. Karmakar, H. B. Li, J. M. Li, J. Li, Q. Y. Li, R. M. J. Li, X. Q. Li, Y. L. Li, Y. F. Liang, B. Liao, F. K. Lin, S. T. Lin, J. X. Liu, S. K. Liu, Y. D. Liu, Y. Liu, Y. Y. Liu, Z. Z. Liu, H. Ma, Y. C. Mao, Q. Y. Nie, J. H. Ning, H. Pan, N. C. Qi, J. Ren, X. C. Ruan, Z. She, M. K. Singh, T. X. Sun, C. J. Tang, W. Y. Tang, Y. Tian, G. F. Wang, L. Wang, Q. Wang, Y. F. Wang, Y. X. Wang, H. T. Jia, S. Y. Wu, Y. C. Wu, H. Y. Xing, R. Xu, Y. Xu, T. Xue, Y. L. Yan, N. Yi, C. X. Yu, H. J. Yu, J. F. Yue, M. Zeng, Z. Zeng, B. T. Zhang, F. S. Zhang, L. Zhang, Z. H. Zhang, Z. Y. Zhang, K. K. Zhao, M. G. Zhao, J. F. Zhou, Z. Y. Zhou, J. J. Zhu, Y. C. Wu

Summary: We investigate exotic neutrino interactions using data from the CDEX-10 experiment at the China Jinping Underground Laboratory. New constraints on the mass and couplings of new gauge bosons are presented. Two nonstandard neutrino interactions involving a UO1 thorn B-L gauge boson and a dark photon are considered.

PHYSICAL REVIEW D (2023)

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Article Chemistry, Multidisciplinary

The sequential structural transformation of a heptanuclear zinc cluster towards hierarchical porous carbon for supercapacitor applications

Tian Li, Yi-Fan Wang, Zheng Yin, Jian Li, Xu Peng, Ming-Hua Zeng

Summary: This study investigated the effects of cluster packing modes on phase and morphological changes during pyrolysis, revealing that weak correlative interactions and shape matching play important roles. The tracking of the pyrolysis process showed changes in solid material composition and porosity. Micro-mesoporous carbon Zn-7-1000 exhibited high capacitance and specific surface area, making it a potential candidate for high-performance devices.

CHEMICAL SCIENCE (2022)

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Article Chemistry, Organic

Ruthenium-catalyzed meta-difluoromethylation of arene phosphines enabled by 1,3-dione

Wen-Qian Xu, Jun-Yang Tao, Yue-Jin Liu, Ming-Hua Zeng

Summary: A highly efficient ruthenium-catalyzed difluoromethylation of arene phosphines has been developed using 1,3-dione as an effective ligand. A wide range of biarylphosphines with various functional groups are compatible with the reaction conditions, affording meta-difluoromethylated phosphine products in moderate to good yields.

ORGANIC CHEMISTRY FRONTIERS (2022)

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Article Chemistry, Physical

Electronic structures of hydroxylated low index surfaces of rutile and anatase-type titanium dioxide

Lu Wu, Jin Lin, Linyuan Ren, Qianni Li, Xin Chi, Ling Luo, Yuexing Zhang, Ming-Hua Zeng

Summary: Different surface planes of various types of titanium dioxide crystals have diverse effects on the splitting of H2O and H-2, as well as the electronic structures of hydroxylated titanium dioxide. Particularly, the electronic structures of R-101, R-001, A-110, A-100, and A-001 surfaces are significantly influenced by hydroxylation.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2022)

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