期刊
LASER & PHOTONICS REVIEWS
卷 9, 期 6, 页码 682-688出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/lpor.201500137
关键词
Nanoantenna; whispering-gallery modes; palladium nanorods; free-space coupling; hydrogen sensors
资金
- National Natural Science Foundation of China [11304202, 11434005]
- Natural Science Foundation of Shanghai [13ZR1458000]
- National Key Scientific Instrument Project [2012YQ150092]
- National Basic Research Program of China [2011CB808105]
Due to the broad scattering spectral profiles, localized surface plasmon resonances (LSPRs) of Pd nanoparticles have low resolution and limited sensitivity for hydrogen detection. In this work, we use a simple light-irradiation method to demonstrate that free-space light can be efficiently coupled into and from the microfiber whispering-gallery modes (WGMs) by the Pd nanoantennas. The nanoantenna-microfiber cavity system provides strong intermodal coupling between LSPRs and WGMs, and induces significant modulation of the scattering spectra. A measured full width at half-maximum of 3.2 nm at 622.7 nm is obtained, which is the narrowest in Pd nanoparticle-based LSPR structures reported up to now. The ultranarrow resonances offer enhanced sensitivity to hydrogen gas detection with a figure of merit reaching similar to 2.22. Other advantages of the Pd nanoantenna-microfiber cavity system including independence of precise alignment of excitation light, large tunability of the resonant wavelengths, easy and low-cost fabrication of the system, have also been demonstrated.
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