期刊
CHEMICAL COMMUNICATIONS
卷 48, 期 7, 页码 982-984出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc16360h
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资金
- Grants-in-Aid for Scientific Research [23659008, 24659006, 23390006, 23790012] Funding Source: KAKEN
The first catalytic version of hypervalent aryl-lambda(3)-iodane-induced Hofmann rearrangement of primary carboxamides, which probably involves in situ generation of a tetracoordinated bis(aqua)(hydroxy)phenyl-lambda(3)-iodane complex as an active oxidant from a catalytic amount of iodobenzene by the reaction with m-chloroperbenzoic acid in the presence of HBF4 in dichloromethane-water under mild conditions, was developed.
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